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Optica Publishing Group
  • 14th International Conference on Ultrafast Phenomena
  • Technical Digest (CD) (Optica Publishing Group, 2004),
  • paper ME11

A unified analysis of ultrafast vibrational and orientational dynamics of HOD in D2O

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Broadband infrared spectroscopy measures the ensemble-averaged vibrational dephasing, lifetime, and orientational dynamics of the OH stretch of HOD in D2O. Two-dimensional infrared spectroscopy probes spectral heterogeneity, revealing a slight frequency dependence to spectral diffusion.

© 2004 Optical Society of America

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