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Direct Probing of the Local Solvent Response During Intermolecular Electron Transfer

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Abstract

Following resonant photo-excitation of coumarin 152 in the electron donating solvents aniline and dimethylaniline, dramatic changes the local intermolecular solvent response are monitored directly as a function of time during intermolecular electron transfer using third-order non-resonant Raman spectroscopy.

© 2006 Optical Society of America

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