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Intermolecular communication and a vibrationally adiabatic basis treatment of small-molecule dynamics in low temperature solids

Craig T. Chapman, Jeffrey A. Cina, and Mary A. Rohrdanz

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Abstract

We investigate intermolecular communication between a Ca atom and an I2 molecule in a cryogenic Ar matrix. An adiabatic-basis approach to simulating ultrafast spectroscopic signals from small, matrix-isolated molecules is also presented.

© 2006 Optical Society of America

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