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Ultrafast Optical Nonlinearities of Metal Nanoparticles: Single-Particle Measurements and Correlation to Structure

Norbert F. Scherer, Matthew Pelton, Rongchao Jin, Justin E. Jureller, Mingzhao Liu, Hee Y. Kim, Sungnam Park, and Philippe Guyot-Sionnest

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Abstract

We have measured nonlinear scattering from plasmons in individual Au nanorods and have correlated second-harmonic activity of Ag nanoparticles and clusters to morphology. The measurements reveal novel ultrafast nonlinear phenomena related to electron confinement.

© 2006 Optical Society of America

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