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Conserving Optical Coherence through the Conical Intersection during Retinal Isomerization in Bacteriorhodopsin

Valentyn I. Prokhorenko, Alexei Halpin, Leonid S. Brown, and R.J. Dwayne Miller

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Abstract

Two-dimensional photon-echo electronic spectroscopy of retinal isomerization in bacteriorhodopsin allows tracking the dynamics of the reaction coordinate. Optically induced coherence still persists even after 5 ps, where no excited-state population of the initial isomer is present.

© 2010 Optical Society of America

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