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Initial relaxation dynamics of retinal protonated Schiff-bases determined by Pump Degenerate Four Wave Mixing

Tiago Buckup, Jan P. Kraack, and Marcus Motzkus

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Abstract

Initial relaxation-dynamics of photo-excited all-trans retinal protonated Schiff-bases were investigated with Pump-Degenerate Four Wave Mixing. It is presented that low-frequency modes are excitable only within a short time of relaxation from the Franck-Condon point.

© 2010 Optical Society of America

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