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Deciphering Excited State Evolution in Halorhodopsin with Stimulated Emission Pumping

Oshrat Bismuth, Pavel Komm, Noga Friedman, Tamar Eliash, Mordechai Sheves, and Sanford Ruhman

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Abstract

Femtosecond pump, NIR dump experiments demonstrate that contrary to previous reports, nonexponential internal conversion in Natronomonas pharaonis Halorhodopsin doesn’t reflect bifurcation in the fluorescent state to short lived reactive, and slowly decaying non reactive populations.

© 2010 Optical Society of America

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