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The First Picoseconds in the Life of Benzhydryl Cations: Ultrafast Generation and Chemical Reactions

Christian F. Sailer, Benjamin P. Fingerhut, Johannes Ammer, Christoph Nolte, Igor Pugliesi, Herbert Mayr, Regina de Vivie-Riedle, and Eberhard Riedle

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Abstract

For benzhydryl chloride compounds we observe that photodissociation only leads to radical pairs. The typically observed cations are formed by subsequent electron transfer. Reactions of cations in neat alcohols can then occur within 2.6 ps.

© 2010 Optical Society of America

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