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Coherent Control of Multidimensional Nonlinear Optical Signals with Shaped Laser Pulses

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Abstract

Multidimensional nonlinear optical signals with shaped laser pulses are simulated using closed-form expressions that contain pulse envelopes. Multiparameter coherent control using linear and higher-order chirp is applied to photosynthetic excitons to enhance weak cross peaks.

© 2010 Optical Society of America

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