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Selective nonlinear response-preparation in the electronic ground-state by means of Degenerate Four-Wave-Mixing

J. P. Kraack, T. Buckup, and M. Motzkus

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Abstract

Femtosecond Degenerate Four-Wave-Mixing was employed to selectively prepare vibrational coherence-dynamics in electronic ground-states of bio-physically active chromophores. The method can be used to determine pure vibrational coherence evolution in the ground-state.

© 2010 Optical Society of America

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