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Ultrafast vibrational dynamics of water at a zwitterionic lipid/water interface revealed by two-dimensional heterodyne-detected vibrational sum frequency generation (2D HD-VSFG)

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Abstract

2D HD-VSFG is applied to the study of ultrafast vibrational dynamics at a zwitterionic lipid/water interface for the first time. The 2D spectrum reveals spectral diffusion of three distinct water species existing at the interface.

© 2014 Optical Society of America

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