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Coherent Control of the Photodissociation of Triiodide in Solution Reveals New Pathways

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Abstract

We demonstrate control of the photodissociation of triiodide, solvated in ethanol, via phase-shaped UV pulses. The second-order chirp dependence of the diiodide yield hints at additional pathways involving higher-lying potential energy surfaces.

© 2014 Optical Society of America

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