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Preferential Solvation of a Rhenium Photocatalyst Facilitates Ultrafast Intermolecular Electron Transfer

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Abstract

Equilibrium 2D IR spectroscopy was used to measure spectral diffusion of the photo-catalyst Re(bpy)(CO)3Cl in multiple TEOA/solvent mixtures. The spectral diffusion was slowest at the 20%/80% TEOA/solvent (v/v) ratio, indicating occurrence of preferential solvation.

© 2016 Optical Society of America

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More Like This
Electronic Ground and Excited State Spectral Diffusion of a Photocatalyst

Laura M. Kiefer, John T. King, and Kevin J. Kubarych
07.Mon.P1.28 International Conference on Ultrafast Phenomena (UP) 2014

Ultrafast Dynamics in Intermolecular Electron Transfer

Keitaro Yoshihara, Haridas Pal, Hideaki Shirota, Yutaka Nagasawa, and Keisuke Tominaga
ThA.6 International Conference on Ultrafast Phenomena (UP) 1996

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C. Gahl, U. Bovensiepen, C. Frischkorn, and M. Wolf
ThC1 International Conference on Ultrafast Phenomena (UP) 2002

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