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Onset Times in Time-Resolved Photoelectron Spectra to Measure Ultrafast Non-Adiabatic Dynamics in Small Molecular Systems

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Abstract

Using signal onset times, time-resolved photoelectron kinetic energy spectra from a two VUV photon pump-probe scheme allow for the tracking of ultrafast (<10 fs) non-adiabatic dynamics of valence excited molecules.

© 2016 Optical Society of America

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