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Superatom State-Resolved Dynamics of Structurally Precise Clusters from Two-Dimensional Electronic Spectroscopy

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Abstract

Femtosecond two-dimensional electronic spectroscopy was used to investigate Superatom electronic dynamics of structurally precise Au25(SC8H9)18 monolayer-protected clusters. Quantification of time-dependent cross-peaks distinguished dynamics of the superatom P and D states with approximate 10-fs time resolution.

© 2016 Optical Society of America

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