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Molecular dissociation driven by plasmonic near-fields of shaped mid-infrared pulses: Impact of down-chirping

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Abstract

We demonstrate vibrationally-mediated dissociation of condensed-phase molecules by employing intense plasmonic near-fields of temporally-shaped mid-infrared pulses. Furthermore, we numerically investigate the impact of down-chirping on the plasmon-enhanced vibrational ladder climbing. © 2020 The Author(s)

© 2020 The Author(s)

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