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Intramolecular charge transfer state of “push-pull” dyes probed by femtosecond stimulated Raman spectroscopy

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Two distinct Raman spectra of “push-pull” dyes, DCM and LD 688, in the locally-excited and charge-transfer states separately obtained from time-resolved Raman measurements, showed the existence of twist intramolecular charge transfer state in polar solvents.

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