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Implementation of Broadband near-UV Pump Pulses for Ultrafast 2D Electronic-Vibrational Spectroscopy

Jason W. Sandwisch, James D. Gaynor, and Munira Khalil

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Abstract

We present the generation of efficient, tunable sub-20 fs broadband near UV pulses. The tunable pulses are used in two-dimensional electronic-vibrational spectroscopy and reveal additional vibronic states in an excited state intramolecular proton transfer process.

© 2020 The Author(s)

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