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Coherently and Fluorescence-Detected Four- and Six-Wave-Mixing Two-Dimensional Electronic Spectroscopy: Measuring Multi-Exciton Dynamics and Delocalization

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Abstract

We directly compare nonlinear coherently and fluorescence-detected two-dimensional electronic spectra of electronically coupled squaraine heterodimers. By identifying signatures of multi-exciton nonequilibrium dynamics and delocalization, we establish grounds for interpretation of these nonlinear spectroscopy implementations.

© 2020 The Author(s)

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