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Direct Visualization of Polaron Formation in the Thermoelectric SnSe

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Abstract

Using ultrafast electron scattering we directly observe the bimodal and anisotropic lattice distortions that drive carrier localization in SnSe. Large (18.7 Å), quasi-1D polarons form in 300 fs and smaller (4.2 Å) 3D polarons form in 4 ps.

© 2022 The Author(s)

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