Revealing the Geometric Phase Effects Around Conical Intersections in Molecules by High-order Harmonic Spectroscopy

Guanglu Yuan; Shicheng Jiang; Ruifeng Lu; Ruifeng Lu; Konstantin Dorfman

doi:10.1364/UP.2022.M2A.2

The International Conference on Ultrafast Phenomena (UP) 2022
Technical Digest Series (Optica Publishing Group, 2022),
paper M2A.2
•https://doi.org/10.1364/UP.2022.M2A.2

Revealing the Geometric Phase Effects Around Conical Intersections in Molecules by High-order Harmonic Spectroscopy

Guanglu Yuan, Shicheng Jiang, Ruifeng Lu, and Konstantin Dorfman

International Conference on Ultrafast Phenomena 2022

Montreal, Quebec Canada
18–22 July 2022
ISBN: 978-1-957171-07-4

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Femtochemistry (M2A)

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G. Yuan, S. Jiang, R. Lu, and K. Dorfman, "Revealing the Geometric Phase Effects Around Conical Intersections in Molecules by High-order Harmonic Spectroscopy," in The International Conference on Ultrafast Phenomena (UP) 2022, F. Légaré, T. Tahara, J. Biegert, T. Brixner, and N. Dudovich, eds., Technical Digest Series (Optica Publishing Group, 2022), paper M2A.2.

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Abstract

We theoretically established a multi-potential energy surface model of the molecule under the diabatic representation, and proposed a scheme to probe the geometric phase effect around the conical intersection by using high-order harmonic spectroscopy.

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