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Time-Resolved Electron and Hole Transfer Dynamics in a TMD Heterostructure by Two-Dimensional Electronic Spectroscopy

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Abstract

Photoexcited electrons and holes rapidly undergo spatial separation in transition metal dichalcogenide Heterostructures (HS) with Type II band alignment. Using Two-dimensional Electronic Spectroscopy, we simultaneously detect interlayer hole and electron transfer in a WS2/MoS2 HS with sub-100 fs timescales.

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