From Femtosecond Excited-State and Dissociation Dynamics to Nanosecond Reaction Kinetics: Following C-H Bond Activation with X-rays

Raphael M. Jay; Ambar Banerjee; Torsten Leitner; Robert Stefanuik; Ru-Pan Wang; Jessica Harich; Emma Beale; Victoria Kabanova; Abdullah Kahraman; Anna Wach; Dimitri Ozerov; Christopher A. Arrell; Philip J. M. Johnson; Grigory Smolentsev; Thomas Huthwelker; Camilia N. Borca; Claudio Cirelli; Camila Bacellar; Christopher J. Milne; Nils Huse; Michael Odelius; Philippe Wernet

doi:10.1364/UP.2022.Tu1A.2

The International Conference on Ultrafast Phenomena (UP) 2022
Technical Digest Series (Optica Publishing Group, 2022),
paper Tu1A.2
•https://doi.org/10.1364/UP.2022.Tu1A.2

From Femtosecond Excited-State and Dissociation Dynamics to Nanosecond Reaction Kinetics: Following C-H Bond Activation with X-rays

Raphael M. Jay, Ambar Banerjee, Torsten Leitner, Robert Stefanuik, Ru-Pan Wang, Jessica Harich, Emma Beale, Victoria Kabanova, Abdullah Kahraman, Anna Wach, Dimitri Ozerov, Christopher A. Arrell, Philip J. M. Johnson, Grigory Smolentsev, Thomas Huthwelker, Camilia N. Borca, Claudio Cirelli, Camila Bacellar, Christopher J. Milne, Nils Huse, Michael Odelius, and Philippe Wernet

International Conference on Ultrafast Phenomena 2022

Montreal, Quebec Canada
18–22 July 2022
ISBN: 978-1-957171-07-4

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Dynamics of Complex Molecular Systems (Tu1A)

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R. M. Jay, A. Banerjee, T. Leitner, R. Stefanuik, R. Wang, J. Harich, E. Beale, V. Kabanova, A. Kahraman, A. Wach, D. Ozerov, C. A. Arrell, P. J. M. Johnson, G. Smolentsev, T. Huthwelker, C. N. Borca, C. Cirelli, C. Bacellar, C. J. Milne, N. Huse, M. Odelius, and P. Wernet, "From Femtosecond Excited-State and Dissociation Dynamics to Nanosecond Reaction Kinetics: Following C-H Bond Activation with X-rays," in The International Conference on Ultrafast Phenomena (UP) 2022, F. Légaré, T. Tahara, J. Biegert, T. Brixner, and N. Dudovich, eds., Technical Digest Series (Optica Publishing Group, 2022), paper Tu1A.2.

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Abstract

Using ultrafast X-ray absorption spectroscopy, we observe how a rhodium carbonyl catalyst is formed on femtosecond timescales and reveal the decisive orbital interactions which facilitate the efficient cleavage of an alkane C-H bond from solution.

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