Breaking the electronic-optical dynamics correspondence via non-perturbative nonlinearities in ultrafast plasmonics

Andrea Schirato; Andrea Schirato; Giulia Crotti; Giulia Crotti; Mychel Gonçalves Silva; Danielle C. Teles-Ferriera; Cristian Manzoni; Remo Proietti Zaccaria; Remo Proietti Zaccaria; Paolo Laporta; Paolo Laporta; Ana Maria de Paula; Giulio Cerullo; Giulio Cerullo; Giuseppe Della Valle; Giuseppe Della Valle; Giuseppe Della Valle

doi:10.1364/UP.2022.W2A.5

The International Conference on Ultrafast Phenomena (UP) 2022
Technical Digest Series (Optica Publishing Group, 2022),
paper W2A.5
•https://doi.org/10.1364/UP.2022.W2A.5

Breaking the electronic-optical dynamics correspondence via non-perturbative nonlinearities in ultrafast plasmonics

Andrea Schirato, Giulia Crotti, Mychel Gonçalves Silva, Danielle C. Teles-Ferriera, Cristian Manzoni, Remo Proietti Zaccaria, Paolo Laporta, Ana Maria de Paula, Giulio Cerullo, and Giuseppe Della Valle

International Conference on Ultrafast Phenomena 2022

Montreal, Quebec Canada
18–22 July 2022
ISBN: 978-1-957171-07-4

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Ultrafast Spectroscopy II (W2A)

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A. Schirato, G. Crotti, M. G. Silva, D. C. Teles-Ferriera, C. Manzoni, R. P. Zaccaria, P. Laporta, A. M. de Paula, G. Cerullo, and G. D. Valle, "Breaking the electronic-optical dynamics correspondence via non-perturbative nonlinearities in ultrafast plasmonics," in The International Conference on Ultrafast Phenomena (UP) 2022, F. Légaré, T. Tahara, J. Biegert, T. Brixner, and N. Dudovich, eds., Technical Digest Series (Optica Publishing Group, 2022), paper W2A.5.

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Abstract

We combine hot-electron dynamical modelling and ultrafast transient absorption spectroscopy to investigate the onset of non-perturbative effects of optical nonlinearities in plasmonic nanostructures, breaking the correspondence between dynamics of optical signal and photoexcited hot carriers.

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