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Femtometer-precision vibrational metrology in molecules with TR-XAS

Patrick Rupprecht, Lennart Aufleger, Simon Heinze, Alexander Magunia, Thomas Ding, Marc Rebholz, Stefano Amberg, Nikola Mollov, Felix Henrich, Maurits Haverkort, Christian Ott, and Thomas Pfeifer

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Abstract

We measure the perturbatively excited symmetric breathing mode vibration A1g in SF6 via time-resolved x-ray absorption spectroscopy. Vibrational amplitudes of 50 fm were resolved. An ab-initio simulation confirms the results and reveals additional electronic coupling.

© 2022 The Author(s)

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