Remote detection of pollutants using resonance Raman scattering

H. Rosen; P. Robrish; O. Chamberlain

doi:10.1364/AO.14.002703

Applied Optics
Vol. 14,
Issue 11,
pp. 2703-2706
(1975)
•https://doi.org/10.1364/AO.14.002703

Remote detection of pollutants using resonance Raman scattering

H. Rosen, P. Robrish, and O. Chamberlain

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H. Rosen, P. Robrish, and O. Chamberlain, "Remote detection of pollutants using resonance Raman scattering," Appl. Opt. 14, 2703-2706 (1975)

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Abstract

Calculations of the resonance Raman cross section for several diatomic molecules are presented. These results are used, together with recent measurements of large resonance enhancements in NO₂ and SO₂, to estimate the sensitivity of a lidar system based upon the resonance Raman effect.

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Molecule	Electronic transition	Vibrational transition	λ_L (Å)	$\frac{d σ}{d Ω} {({cm}^{2} / sr)}_{calc .}$	$\frac{d σ}{d Ω} {({cm}^{2} / sr)}_{exp .}$	Refs.
CO⁺	A²Π_i − X²Σ⁺	0-1, 1-1	4913	2.5 × 10⁻²⁰		16
SO	A³Π₀ − X³Σ⁻	0-2, 2-0	2579	1.3 × 10⁻²⁰		17
OH	A²Σ⁺ − X³Π_i	0-0, 0-1	3064	2.4 × 10⁻²²	10⁻²⁰ to 10⁻²¹ (Ref. 11)	18, 19
NO	A²Σ⁺ − X²Π	0-0, 0-3	2262	1.3 × 10⁻²³		20, 21
I₂	B³Π_Ou⁺ − X¹Σ_g⁺	0-25, 25-1	5466.36	1.2 × 10⁻²⁴	1.7 × 10⁻²⁴	9, 22, 23
SO₂	$Ã ({{}^{1}B}_{1}) - {\tilde{X}}^{1} A_{1}$		2999.6		1 × 10⁻²⁵	2
79_Br81_Br	B³Π_Ou⁺ − X¹Σ_g⁺	0-28, 28-1	5264.0	7.8 × 10⁻²⁷		24, 25
NO₂	$Ã ({{}^{2}B}_{1}) - {\tilde{X}}^{2} A_{1} (?)$		4547.4		5.6 × 10⁻²⁷	1
CO	a³Π − X¹Σ⁺	0-0, 0-1	2063	4.5 × 10⁻³⁰		16
Cl₂	A³Π_Ou⁺ − X¹Σ_g⁺	0-15, 15-3	4933	7 × 10⁻³¹		24, 26

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Applied Optics