Multiphoton fragmentation and ionization

M. B. Robin

doi:10.1364/AO.19.003941

Applied Optics
Vol. 19,
Issue 23,
pp. 3941-3947
(1980)
•https://doi.org/10.1364/AO.19.003941

Multiphoton fragmentation and ionization

M. B. Robin

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M. B. Robin, "Multiphoton fragmentation and ionization," Appl. Opt. 19, 3941-3947 (1980)

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Abstract

This paper discusses the complications of postresonant processes in the ionization pathways and their effects on the polarization ratio and the power laws for various ionic fragments, using acetaldehyde and nitrogen dioxide as examples.

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Fragment	Species	(λ+ρ+ρ₀)N_i(T)/ρN_gT
CH₃CHO⁺	1	$\begin{array}{l} σ_{r 1} I & - \frac{1}{2} {T σ}_{r 1} (σ_{12} + σ_{13} + σ_{14}) I^{2} - \frac{1}{2} {T σ}_{r 1} (σ_{12}^{'} \\ + σ_{13}^{'} + σ_{14}^{'} + σ_{15}^{'} σ_{16}^{'}) I^{3} \end{array}$ ^a
CH₃CO⁺	2	$(σ_{r 2} + \frac{1}{2} {T σ}_{r 1} σ_{12}) I^{2} + \frac{1}{2} {T σ}_{r 1} σ_{12}^{'} I^{3}$
CHO⁺	3	$(σ_{r 3} + \frac{1}{2} {T σ}_{r 1} σ_{13}) I^{2} + \frac{1}{2} {T σ}_{r 1} σ_{13}^{'} I^{3}$
${CH}_{4}^{+}$	4	$\begin{array}{l} (σ_{r 4} & + \frac{1}{2} {T σ}_{r 1} σ_{14}) I^{2} + \frac{1}{2} T [σ_{r 1} σ_{14}^{'} - σ_{r 4} (σ_{45} \\ + σ_{46})] I^{3} \end{array}$
${CH}_{3}^{+}$	5	$(σ_{r 5} + \frac{1}{2} {T σ}_{r 1} σ_{15}^{'} + \frac{1}{2} {T σ}_{r 4} σ_{45}) I^{3}$
${CH}_{2}^{+}$	6	$\begin{array}{l} (σ_{r 6} & + \frac{1}{2} {T σ}_{r 6} σ_{16}^{'} + \frac{1}{2} {T σ}_{r 4} σ_{46}) I^{3} \\ - \frac{1}{2} {T σ}_{r 6} σ_{6 x} I^{4} \end{array}$ ^b

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Applied Optics