Crystal structure dependence of the breathing vibration of individual gold nanodisks induced by the ultrafast laser

Yong Gan; Zheng Sun

doi:10.1364/AO.58.000213

Applied Optics
Vol. 58,
Issue 1,
pp. 213-218
(2019)
•https://doi.org/10.1364/AO.58.000213

Crystal structure dependence of the breathing vibration of individual gold nanodisks induced by the ultrafast laser

Yong Gan and Zheng Sun

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Yong Gan and Zheng Sun, "Crystal structure dependence of the breathing vibration of individual gold nanodisks induced by the ultrafast laser," Appl. Opt. 58, 213-218 (2019)

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Table of Contents Category
- Lasers, Optical Amplifiers, and Laser Optics
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About this Article
History
- Original Manuscript: October 18, 2018
- Revised Manuscript: November 28, 2018
- Manuscript Accepted: November 29, 2018
- Published: December 21, 2018

Abstract

The ultrafast laser-excited breathing vibrations of gold nanodisks with different crystal structures have been studied via atomistic simulations. The vibrational periods and damping rates of nanodisks are obtained by the analysis of the simulated transient responses of nanodisks. It is shown that the breathing period of nanodisks is considerably dependent on their crystal structure, which is contrary to the cases for the breathing vibration of metal nanospheres and nanorods. Furthermore, single-crystal nanodisks exhibit much lower intrinsic damping as compared with polycrystalline nanodisks, for which the additional energy dissipation by the grain boundaries in the polycrystalline nanodisks could be one major factor.

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Elastic Constants	Ref. [25]	Ref. [27]	Ref. [28]	Experiment [29]
$c_{11}$ (GPa)	198.89	172.23	209.65	192.34
$c_{12}$ (GPa)	165.88	151.47	176.44	163.14
$c_{44}$ (GPa)	38.29	40.31	46.13	41.95

Nanodisk	Diameter (nm)	Thickness (nm)	Breathing Period $T_{br}$ (ps)
$G_{s}$	$781.915 \pm 0.004$	$162.240 \pm 0.121$	$63.518 \pm 0.004$
$G_{3}$	$780.022 \pm 0.153$	$164.637 \pm 0.231$	$60.648 \pm 0.114$
$G_{10}$	$780.305 \pm 0.1$	$164.932 \pm 0.076$	$53.842 \pm 0.112$

Nanodisk	$τ$ (ps)	Quality Factor $Q$
$G_{s}$	$1971.4 \pm 35.7$	$97.5 \pm 1.8$
$G_{3}$	$715.1 \pm 42.0$	$37.0 \pm 2.2$
$G_{10}$	$530.2 \pm 42.9$	$30.9 \pm 2.5$

Elastic Constants	Ref. [25]	Ref. [27]	Ref. [28]	Experiment [29]
$c_{11}$ (GPa)	198.89	172.23	209.65	192.34
$c_{12}$ (GPa)	165.88	151.47	176.44	163.14
$c_{44}$ (GPa)	38.29	40.31	46.13	41.95

Nanodisk	Diameter (nm)	Thickness (nm)	Breathing Period $T_{br}$ (ps)
$G_{s}$	$781.915 \pm 0.004$	$162.240 \pm 0.121$	$63.518 \pm 0.004$
$G_{3}$	$780.022 \pm 0.153$	$164.637 \pm 0.231$	$60.648 \pm 0.114$
$G_{10}$	$780.305 \pm 0.1$	$164.932 \pm 0.076$	$53.842 \pm 0.112$

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Applied Optics