Nonlinear optical limiting effect of graphene dispersions at 1064 nm

Youwen Xie; Youwen Xie; Yuangang Lu; Yuangang Lu; Jian Huang; Zhengnan Wu; Zhengnan Wu; Feng Xu; Dunwen Zuo

doi:10.1364/AO.434978

Applied Optics
Vol. 60,
Issue 28,
pp. 8858-8864
(2021)
•https://doi.org/10.1364/AO.434978

Nonlinear optical limiting effect of graphene dispersions at 1064 nm

Youwen Xie, Yuangang Lu, Jian Huang, Zhengnan Wu, Feng Xu, and Dunwen Zuo

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Youwen Xie, Yuangang Lu, Jian Huang, Zhengnan Wu, Feng Xu, and Dunwen Zuo, "Nonlinear optical limiting effect of graphene dispersions at 1064 nm," Appl. Opt. 60, 8858-8864 (2021)

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Abstract

We study the nonlinear optical limiting effect of graphene dispersions in ethanol and acetone at a wavelength of 1064 nm. The nonlinear optical limiting effect of graphene dispersion under three different linear transmittances (about 70%, 80%, and 90%), two different thicknesses (1 and 3 cm), and two different solvents (ethanol and acetone) are measured. The influences of concentration, thickness, and solvent on the nonlinear optical limiting effect of the graphene dispersion are analyzed. The experimental results show that the concentration and solution thicknesses have great influence on the optical limiting ability of graphene dispersions. The graphene dispersions with ethanol and acetone as solvents can be used to achieve excellent nonlinear optical limiting effects. The optical limiting ability of the graphene dispersion in acetone is better than that of the graphene dispersion in ethanol.

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Data underlying the results presented in this paper are not publicly available at this time but may be obtained from the authors upon reasonable request.

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Number	Concentration (mg/mL)	Solvent	$N_{e f f}$	$T_{0}$
1	0.0044	Ethanol	$8.84 * 10^{7}$	71.3%
2	0.0025	Ethanol	$4.97 * 10^{7}$	79.9%
3	0.0007	Ethanol	$1.42 * 10^{7}$	90.3%
4	0.0080	Acetone	$1.59 * 10^{8}$	67.6%
5	0.0040	Acetone	$7.96 * 10^{7}$	78.5%
6	0.0020	Acetone	$3.98 * 10^{7}$	90.6%

Solvent	Concentration (mg/mL)	Thickness (cm)	$T_{0}$	$δ$	$T_{min}$
Ethanol	0.0007	1	90.3%	0.316	58.7%
	0.0007	3	63.5%	0.477	15.8%
	0.0025	1	79.9%	0.501	29.8%
	0.0025	3	53.5%	0.405	13.0%
	0.0044	1	71.3%	0.534	17.9%
	0.0044	3	32.3%	0.285	3.8%
Acetone	0.0020	1	90.6%	0.528	37.8%
	0.0020	3	77.8%	0.575	20.3%
	0.0040	1	78.5%	0.531	25.4%
	0.0040	3	62.1%	0.501	12.0%
	0.0080	1	67.6%	0.521	15.5%
	0.0080	3	27.6%	0.232	4.4%

Material	$δ$	$T_{min}$	References
Graphene in acetone at 1064 nm	0.575	0.203	This paper
Graphene in ethanol at 1064 nm	0.534	0.179	This paper
Graphene in N-methyl-2-pyrrolidone at 1064 nm	0.201	0.603	[9]
Graphene in N,N-dimethylacetamide at 1064 nm	0.236	0.552	[9]
Graphene in $γ$ -butyrolactone at 1064 nm	0.162	0.648	[9]
Graphene in ethanol at 532 nm	0.400	0.200	[16]
$C_{70}$ in toluene at 1064 nm	0.480	0.320	[23]
DWNT– $C_{60}$ in chlorobenzene PmPV/toluene at 532 nm	0.520	0.280	[24]
Graphene/ZnO hybrid organic glasses at 532 nm	0.344	0.317	[25]
Graphene oxide nanoribbons at 1064 nm	0.385	0.315	[26]
Cu nanowires at 1064 nm	0.310	0.580	[27]

Number	Concentration (mg/mL)	Solvent	$N_{e f f}$	$T_{0}$
1	0.0044	Ethanol	$8.84 * 10^{7}$	71.3%
2	0.0025	Ethanol	$4.97 * 10^{7}$	79.9%
3	0.0007	Ethanol	$1.42 * 10^{7}$	90.3%
4	0.0080	Acetone	$1.59 * 10^{8}$	67.6%
5	0.0040	Acetone	$7.96 * 10^{7}$	78.5%
6	0.0020	Acetone	$3.98 * 10^{7}$	90.6%

Solvent	Concentration (mg/mL)	Thickness (cm)	$T_{0}$	$δ$	$T_{min}$
Ethanol	0.0007	1	90.3%	0.316	58.7%
	0.0007	3	63.5%	0.477	15.8%
	0.0025	1	79.9%	0.501	29.8%
	0.0025	3	53.5%	0.405	13.0%
	0.0044	1	71.3%	0.534	17.9%
	0.0044	3	32.3%	0.285	3.8%
Acetone	0.0020	1	90.6%	0.528	37.8%
	0.0020	3	77.8%	0.575	20.3%
	0.0040	1	78.5%	0.531	25.4%
	0.0040	3	62.1%	0.501	12.0%
	0.0080	1	67.6%	0.521	15.5%
	0.0080	3	27.6%	0.232	4.4%

Abstract

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Applied Optics