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Color-center laser kinetic spectroscopy: observation of the a1 Δ NH vibrational fundamental

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Abstract

The vibrational fundamental of a1Δ NH formed by 193-nm excimer-laser photolysis of gaseous HN3 has been observed using a color-center laser. The high degree of rotational excitation resulting from the photolysis, corresponding to a temperature of ∼10 000 K, allows high-order centrifugal distortion constants to be determined. The frequencies of the 35 observed lines and the centrifugal distortion constants determined from them are reported.

© 1985 Optical Society of America

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