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Effective nonlinear optical properties of graded metal–dielectric composite films of anisotropic particles

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Abstract

We study the effective third-order nonlinear susceptibility of a graded metal–dielectric composite film of anisotropic particles with weak nonlinearity by invoking the local field effects within the Maxwell–Garnett theory. We further numerically demonstrate that the film can serve as a novel optical material to produce a broad structure in both the linear and the nonlinear response and an enhancement in the nonlinear response.

© 2005 Optical Society of America

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