Abstract
Nonlinear index of refraction of a series of organic solvents, measured by the nonlinear imaging (z-scan) technique, is compared with the same values derived from optical third-harmonic generation (THG). The systematic differences in the values obtained from the z-scan measurements and from THG are attributed to three factors: the value of the standard used in THG measurements, important rotational contribution in z-scan measurements, and the difference in dispersion for derived from Kerr susceptibility and those derived from THG measurements. Using the recently proposed standard silica susceptibility value, one obtains a very good agreement for silica and significant differences for the solvents, particularly for and chlorobenzene. A correction based on a three-level model for centrosymmetric media is applied for dispersion.
© 2008 Optical Society of America
Full Article |
PDF Article
More Like This
References
You do not have subscription access to this journal. Citation lists with outbound citation links are available to subscribers only. You may subscribe either as an Optica member, or as an authorized user of your institution.
Contact your librarian or system administrator
or
Login to access Optica Member Subscription
Cited By
You do not have subscription access to this journal. Cited by links are available to subscribers only. You may subscribe either as an Optica member, or as an authorized user of your institution.
Contact your librarian or system administrator
or
Login to access Optica Member Subscription
Figures (6)
You do not have subscription access to this journal. Figure files are available to subscribers only. You may subscribe either as an Optica member, or as an authorized user of your institution.
Contact your librarian or system administrator
or
Login to access Optica Member Subscription
Tables (3)
You do not have subscription access to this journal. Article tables are available to subscribers only. You may subscribe either as an Optica member, or as an authorized user of your institution.
Contact your librarian or system administrator
or
Login to access Optica Member Subscription
Equations (17)
You do not have subscription access to this journal. Equations are available to subscribers only. You may subscribe either as an Optica member, or as an authorized user of your institution.
Contact your librarian or system administrator
or
Login to access Optica Member Subscription