Abstract

Measurements of the vacuum-ultraviolet (<80-nm) radiation produced by intense ultraviolet (248-nm) irradiation (10¹⁵–10¹⁶ W/cm²) of rare gases have revealed the copious presence of both harmonic radiation and fluorescence from excited levels. The highest harmonic observed was the seventeenth (14.6 nm) in Ne, the shortest wavelength ever produced by that means. Strong fluorescence was seen from ions of Ar, Kr, and Xe, with the shortest wavelengths observed being below 12 nm. Furthermore, radiation from inner-shell excited configurations in Xe, specifically the 4d⁹5s5p → 4d¹⁰5s manifold of Xe⁷⁺ at ~17.7 nm, was detected. These experimental findings, in alliance with other studies concerning multielectron processes, give evidence for a role of electron correlations in a direct nonlinear process of inner-shell excitation.

© 1987 Optical Society of America

Subpicosecond ultraviolet multiphoton electron spectroscopy of rare gases

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