Newly observed lines and hyperfine structure in the infrared spectrum of indium obtained by using a Fourier-transform spectrometer

S. George; G. Guppy; J. Verges

doi:10.1364/JOSAB.7.000249

Journal of the Optical Society of America B
Vol. 7,
Issue 3,
pp. 249-252
(1990)
•https://doi.org/10.1364/JOSAB.7.000249

Newly observed lines and hyperfine structure in the infrared spectrum of indium obtained by using a Fourier-transform spectrometer

S. George, G. Guppy, and J. Verges

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S. George, G. Guppy, and J. Verges, "Newly observed lines and hyperfine structure in the infrared spectrum of indium obtained by using a Fourier-transform spectrometer," J. Opt. Soc. Am. B 7, 249-252 (1990)

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Abstract

The spectrum of neutral indium has been studied in the infrared region by means of the Fourier-transform spectrometer at the Laboratoire Aime Cotton, Orsay, France. A microwave-excited discharge tube containing indium iodide was used as the light source. A total of ten hyperfine structures was studied. Precise measurements of the center of gravity of the structures give energy levels with an error less than 0.005 cm⁻¹. Complete analysis of these hyperfine structures resulted in the determination of the magnetic-dipole and electric-quadrupole interaction constants for one odd and four even levels. The observation also resulted in the measurements of 57 lines in the region of 0.86–4.0 μm, and, of these, 41 lines were observed for the first time to our knowledge.

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Intensity	Wave Number (cm⁻¹)^a	Wavelength (Air; Å)	Classification (Even–Odd; cm⁻¹)
2	2 559.584 cg	39 058.20	$7 s^{2} S_{1 / 2} - 7 p^{2} P_{1 / 2}^{°}$
6	2 671.047 cg	37 428.30	$7 s^{2} S_{1 / 2} - 7 p^{2} P_{3 / 2}^{°}$
1	2 863.510	34 912.67	$7 d^{2} D_{3 / 2} - 7 p^{2} P_{3 / 2}^{°}$
4	2 889.067	34 604.19	$7 d^{2} D_{5 / 2} - 7 p^{2} P_{3 / 2}^{°}$
2	2 974.995	33 604.34	$7 d^{2} D_{3 / 2} - 7 p^{2} P_{1 / 2}^{°}$
21	3 121.817	32 023.90	$6 d^{2} D_{5 / 2} - 5 f^{2} F_{7 / 2}^{°}$
6	3 171.705	31 520.19	$6 d^{2} D_{3 / 2} - 5 f^{2} F_{5 / 2}^{°}$
2	3 746.117	26 687.03	$9 s^{2} S_{1 / 2} - 7 p^{2} P_{3 / 2}^{°}$
2	3 857.588	25 915.87	$9 s^{2} S_{1 / 2} - 7 p^{2} P_{1 / 2}^{°}$
7	3 905.622	25 597.14	$5 p^{24} P_{3 / 2} - 6 p^{2} P_{3 / 2}^{°}$
1427	4 186.614 cg	23 879.12	$7 s^{2} S_{1 / 2} - 6 p^{2} P_{3 / 2}^{°}$
23	4 203.537 cg	23 783.00	$5 p^{24} P_{3 / 2} - 6 p^{2} P_{1 / 2}^{°}$
1	4 363.016	22 913.61	$8 d^{2} D_{3 / 2} - 7 p^{2} P_{3 / 2}^{°}$
7	4 382.197	22 813.42	$8 d^{2} D_{5 / 2} - 7 p^{2} P_{3 / 2}^{°}$
3	4 474.496	22 432.79	$8 d^{2} D_{3 / 2} - 7 p^{2} P_{1 / 2}^{°}$
1145	4 484.882 cg	22 291.00	$7 s^{2} S_{1 / 2} - 6 p^{2} P_{1 / 2}^{°}$
4	4 486.221	22 284.39	$6 d^{2} D_{5 / 2} - 6 f^{2} F_{7 / 2}^{°}$
5	4 536.095	22 039.40	$6 d^{2} D_{3 / 2} - 6 f^{2} F_{5 / 2}^{°}$
1	4 908.400	20 367.68	$10 s^{2} S_{7 / 2} - 7 p^{2} P_{3 / 2}^{°}$
1	5 019.868	19 917.41	$10 s^{2} S_{1 / 2} - 7 p^{2} P_{1 / 2}^{°}$
1	5 261.806	18 999.70	$9 d^{2} D_{3 / 2} - 7 p^{2} P_{3 / 2}^{°}$
2	5 276.918	18 945.28	$9 d^{2} D_{5 / 2} - 7 p^{2} P_{3 / 2}^{°}$
2	5 307.856	18 834.86	$6 d^{2} D_{5 / 2} - 7 f^{2} F_{7 / 2}^{°}$
468	5 336.719 cg	18 732.99	$5 p^{24} P_{5 / 2} - 6 p^{2} P_{3 / 2}^{°}$
2	5 357.723	18 659.55	$6 d^{2} D_{3 / 2} - 7 f^{2} F_{5 / 2}^{°}$
2	5 373.261	18 605.59	$9 d^{2} D_{3 / 2} - 7 p^{2} P_{1 / 2}^{°}$
3	5 525.297	18 093.63	$7 s^{2} S_{1 / 2} - 8 p^{2} P_{3 / 2}^{°}$
10	5 579.593 cg	17 917.56	$7 s^{2} S_{1 / 2} - 8 p^{2} P_{3 / 2}^{°}$
1	5 623.532	17 777.57	$11 s^{2} S_{1 / 2} - 7 p^{2} P_{3 / 2}^{°}$
2	5 840.4	17 114.44	$6 d^{2} D_{5 / 2} - 8 f^{2} F_{7 / 2}^{°}$
1	5 854.564	17 076.03	$10 d^{2} D_{5 / 2} - 7 p^{2} P_{3 / 2}^{°}$
1	5 890.25	16 977.57	$6 d^{2} D_{3 / 2} - 8 f^{2} F_{5 / 2}^{°}$
49	5 969.216	16 748.05	$5 d^{2} D_{3 / 2} - 7 p^{2} P_{1 / 2}^{°}$
78	6 057.370	16 504.30	$5 d^{2} D_{5 / 2} - 7 p^{2} P_{3 / 2}^{°}$
8	6 080.683	16 441.03	$5 d^{2} D_{3 / 2} - 7 p^{2} P_{3 / 2}^{°}$
1731	6 792.083	14 719.10	$5 d^{2} D_{5 / 2} - 4 f^{2} F_{7 / 2}^{°}$
1438	6 815.389	14 668.67	$5 d^{2} D_{3 / 2} - 4 f^{2} F_{5 / 2}^{°}$
241	6 933.325	14 419.15	$6 d^{2} D_{3 / 2} - 6 p^{2} P_{3 / 2}^{°}$
1419	6 983.195	14 316.18	$6 s^{2} D_{5 / 2} - 6 p^{2} P_{3 / 2}^{°}$
972	7 231.594 cg	13 824.43	$6 d^{2} D_{3 / 2} - 6 p^{2} P_{1 / 2}^{°}$
12,241	7 444.026 cg	13 429.93	$6 s^{2} S_{1 / 2} - 6 p^{2} P_{1 / 2}^{°}$
9498	7 742.295 cg	12 912.54	$6 s^{2} S_{1 / 2} - 6 p^{2} P_{3 / 2}^{°}$
24	8 521.748	11 731.47	$8 s^{2} S_{1 / 2} - 6 p^{2} P_{3 / 2}^{°}$
7	8 820.012	11 334.75	$8 s^{2} S_{1 / 2} - 6 p^{2} P_{1 / 2}^{°}$
52	9 304.686	10 744.33	$5 d^{2} D_{5 / 2} - 5 f^{2} F_{7 / 2}^{°}$
38	9 328.052	10 717.42	$5 d^{2} D_{3 / 2} - 5 f^{2} F_{5 / 2}^{°}$
21	9 746.726	10 257.04	$7 d^{2} D_{5 / 2} - 6 p^{2} P_{3 / 2}^{°}$
16	10 019.461	9 977.84	$7 d^{2} D_{3 / 2} - 6 p^{2} P_{1 / 2}^{°}$
1	10 603.776	9 428.02	$9 s^{2} S_{1 / 2} - 6 p^{2} P_{3 / 2}^{°}$
2	19 669.104	9 370.29	$5 d^{2} D_{5 / 2} - 6 f^{2} F_{7 / 2}^{°}$
2	10 692.451	9 349.83	$5 d^{2} D_{3 / 2} - 6 f^{2} F_{5 / 2}^{°}$
1	10 902.049	9 170.07	$9 s^{2} S_{1 / 2} - 6 p^{2} P_{1 / 2}^{°}$
1	11 220.686	8 909.66	$8 d^{2} D_{3 / 2} - 6 p^{2} P_{3 / 2}^{°}$
1	11 239.857	8 894.47	$8 d^{2} D_{5 / 2} - 6 p^{2} P_{3 / 2}^{°}$
1	11 490.7	8 700.30	$5 d^{2} D_{5 / 2} - 7 f^{2} F_{7 / 2}^{°}$
1	11 514.0	8 682.69	$5 d^{2} D_{3 / 2} - 7 f^{2} F_{5 / 2}^{°}$
1	11 518.956	8 678.96	$8 d^{2} D_{3 / 2} - 6 p^{2} P_{1 / 2}^{°}$

Designation	This Paper	Ref. 1	Ref. 25
Odd Configurations
$5 s^{2} (^{1} S) 6 p^{2} P_{1 / 2}^{°}$	31 816.982	31 816.61	31 816.96
${{}^{2}P}_{3 / 2}^{°}$	32 115.251	32 114.79	32 115.22
$5 s^{2} (^{1} S) 7 p^{2} P_{1 / 2}^{°}$	38 861.448	38 861.35	38 861.43
${{}^{2}P}_{3 / 2}^{°}$	38 972.911	38 972.84	38 972.90
$5 s^{2} (^{1} S) 4 f^{2} F_{5 / 2}^{°}$	39 707.161	39 707.29	39 707.59
$F_{7 / 2}^{°}$	39 707.622	39 707.96
$5 s^{2} (^{1} S) 8 p^{2} P_{1 / 2}^{°}$	41 827.167	41 827.10
$5 s^{2} (^{1} S) 8 p^{2} P_{3 / 2}^{°}$	41 881.457	41 881.44
$5 s^{2} (^{1} S) 5 f^{2} F_{5 / 2, 7 / 2}^{°}$	42 220.281	42 220.0	42 220.25
$5 s^{2} (^{1} S) 6 f^{2} F_{5 / 2, 7 / 2}^{°}$	43 584.681	43 584.4	43 584.66
$5 s^{2} (^{1} S) 7 f^{2} F_{5 / 2, 7 / 2}^{°}$	44 406.23	44 406.20(5/2)	44 406.31
		44 406.26(7/2)
$5 s^{2} (^{1} S) 8 f^{2} F_{5 / 2, 7 / 2}^{°}$	44 938.845	44 938.71(5/2)	44 938.81
		44 938.70(7/2)
Even Configurations
5s²(¹S)6s²S_1/2	24 372.956	24 372.87	24 372.956
5s²(¹S)5d²D_3/2	32 892.230	32 892.12	32 892.21
²D_5/2	32 915.539	32 915.42	32 915.54
5s²5p^{2 4}P_3/2	36 020.519	36 020.80
⁴P_5/2	37 451.970	37 451.90
5s²(¹S)7s²S_1/2	36 301.864	36 301.69	36 301.84
5s²(¹S)6d²D_3/2	39 048.576	39 048.48	39 048.53
²D_5/2	39 098.464	39 098.37	39 098.38
5s²(¹S)8s²S_1/2	40 636.996	40 636.71	40 636.98
5s²(¹S)7d²D_3/2	41 836.443	41 836.23	41 836.41
²D_5/2	41 861.978	41 861.57	41 861.96
5s²(¹S)9S²S_1/2	42 719.031	42 718.55	42 719.02
5s²(¹S)8d²D_3/2	43 335.937	43 335.63	43 335.93
²D_5/2	43 355.108	43 354.62	43 354.08
5s²(¹S)10S²S_1/2	43 881.314	43 880.83	43 880.26
5s²(¹S)9d²D_3/2	44 234.704	44 234.26	44 234.70
²D_5/2	44 249.829	44 249.37	44 249.77
5s²(¹S)11S²S_1/2	44 596.443	44 595.86
5s²(¹S)10d²D_5/2	44 827.475	44 827.02

Level	This Paper		Previous Research

	A (mK)	B (mK)	A (mK)	B (mK)	Reference
$6 p^{2} P_{1 / 2}^{°}$	8.35(1)
6s²S_1/2	56.28(2)		56.22(1)^b		14
			56.28(1)^b		13
			56.02(1)^b		18
			56.21(2)^b		16
			55.8		12
			56.17(3)^b		19
5p^{2 4}P_3/2	129.34(82)	−10.03(82)
5p^{2 4}P_5/2	121.93(45)	−21.48(45)
7s²S_1/2	18.05(1)		17.98(4)^b		19

Intensity	Wave Number (cm⁻¹)^a	Wavelength (Air; Å)	Classification (Even–Odd; cm⁻¹)
2	2 559.584 cg	39 058.20	$7 s^{2} S_{1 / 2} - 7 p^{2} P_{1 / 2}^{°}$
6	2 671.047 cg	37 428.30	$7 s^{2} S_{1 / 2} - 7 p^{2} P_{3 / 2}^{°}$
1	2 863.510	34 912.67	$7 d^{2} D_{3 / 2} - 7 p^{2} P_{3 / 2}^{°}$
4	2 889.067	34 604.19	$7 d^{2} D_{5 / 2} - 7 p^{2} P_{3 / 2}^{°}$
2	2 974.995	33 604.34	$7 d^{2} D_{3 / 2} - 7 p^{2} P_{1 / 2}^{°}$
21	3 121.817	32 023.90	$6 d^{2} D_{5 / 2} - 5 f^{2} F_{7 / 2}^{°}$
6	3 171.705	31 520.19	$6 d^{2} D_{3 / 2} - 5 f^{2} F_{5 / 2}^{°}$
2	3 746.117	26 687.03	$9 s^{2} S_{1 / 2} - 7 p^{2} P_{3 / 2}^{°}$
2	3 857.588	25 915.87	$9 s^{2} S_{1 / 2} - 7 p^{2} P_{1 / 2}^{°}$
7	3 905.622	25 597.14	$5 p^{24} P_{3 / 2} - 6 p^{2} P_{3 / 2}^{°}$
1427	4 186.614 cg	23 879.12	$7 s^{2} S_{1 / 2} - 6 p^{2} P_{3 / 2}^{°}$
23	4 203.537 cg	23 783.00	$5 p^{24} P_{3 / 2} - 6 p^{2} P_{1 / 2}^{°}$
1	4 363.016	22 913.61	$8 d^{2} D_{3 / 2} - 7 p^{2} P_{3 / 2}^{°}$
7	4 382.197	22 813.42	$8 d^{2} D_{5 / 2} - 7 p^{2} P_{3 / 2}^{°}$
3	4 474.496	22 432.79	$8 d^{2} D_{3 / 2} - 7 p^{2} P_{1 / 2}^{°}$
1145	4 484.882 cg	22 291.00	$7 s^{2} S_{1 / 2} - 6 p^{2} P_{1 / 2}^{°}$
4	4 486.221	22 284.39	$6 d^{2} D_{5 / 2} - 6 f^{2} F_{7 / 2}^{°}$
5	4 536.095	22 039.40	$6 d^{2} D_{3 / 2} - 6 f^{2} F_{5 / 2}^{°}$
1	4 908.400	20 367.68	$10 s^{2} S_{7 / 2} - 7 p^{2} P_{3 / 2}^{°}$
1	5 019.868	19 917.41	$10 s^{2} S_{1 / 2} - 7 p^{2} P_{1 / 2}^{°}$
1	5 261.806	18 999.70	$9 d^{2} D_{3 / 2} - 7 p^{2} P_{3 / 2}^{°}$
2	5 276.918	18 945.28	$9 d^{2} D_{5 / 2} - 7 p^{2} P_{3 / 2}^{°}$
2	5 307.856	18 834.86	$6 d^{2} D_{5 / 2} - 7 f^{2} F_{7 / 2}^{°}$
468	5 336.719 cg	18 732.99	$5 p^{24} P_{5 / 2} - 6 p^{2} P_{3 / 2}^{°}$
2	5 357.723	18 659.55	$6 d^{2} D_{3 / 2} - 7 f^{2} F_{5 / 2}^{°}$
2	5 373.261	18 605.59	$9 d^{2} D_{3 / 2} - 7 p^{2} P_{1 / 2}^{°}$
3	5 525.297	18 093.63	$7 s^{2} S_{1 / 2} - 8 p^{2} P_{3 / 2}^{°}$
10	5 579.593 cg	17 917.56	$7 s^{2} S_{1 / 2} - 8 p^{2} P_{3 / 2}^{°}$
1	5 623.532	17 777.57	$11 s^{2} S_{1 / 2} - 7 p^{2} P_{3 / 2}^{°}$
2	5 840.4	17 114.44	$6 d^{2} D_{5 / 2} - 8 f^{2} F_{7 / 2}^{°}$
1	5 854.564	17 076.03	$10 d^{2} D_{5 / 2} - 7 p^{2} P_{3 / 2}^{°}$
1	5 890.25	16 977.57	$6 d^{2} D_{3 / 2} - 8 f^{2} F_{5 / 2}^{°}$
49	5 969.216	16 748.05	$5 d^{2} D_{3 / 2} - 7 p^{2} P_{1 / 2}^{°}$
78	6 057.370	16 504.30	$5 d^{2} D_{5 / 2} - 7 p^{2} P_{3 / 2}^{°}$
8	6 080.683	16 441.03	$5 d^{2} D_{3 / 2} - 7 p^{2} P_{3 / 2}^{°}$
1731	6 792.083	14 719.10	$5 d^{2} D_{5 / 2} - 4 f^{2} F_{7 / 2}^{°}$
1438	6 815.389	14 668.67	$5 d^{2} D_{3 / 2} - 4 f^{2} F_{5 / 2}^{°}$
241	6 933.325	14 419.15	$6 d^{2} D_{3 / 2} - 6 p^{2} P_{3 / 2}^{°}$
1419	6 983.195	14 316.18	$6 s^{2} D_{5 / 2} - 6 p^{2} P_{3 / 2}^{°}$
972	7 231.594 cg	13 824.43	$6 d^{2} D_{3 / 2} - 6 p^{2} P_{1 / 2}^{°}$
12,241	7 444.026 cg	13 429.93	$6 s^{2} S_{1 / 2} - 6 p^{2} P_{1 / 2}^{°}$
9498	7 742.295 cg	12 912.54	$6 s^{2} S_{1 / 2} - 6 p^{2} P_{3 / 2}^{°}$
24	8 521.748	11 731.47	$8 s^{2} S_{1 / 2} - 6 p^{2} P_{3 / 2}^{°}$
7	8 820.012	11 334.75	$8 s^{2} S_{1 / 2} - 6 p^{2} P_{1 / 2}^{°}$
52	9 304.686	10 744.33	$5 d^{2} D_{5 / 2} - 5 f^{2} F_{7 / 2}^{°}$
38	9 328.052	10 717.42	$5 d^{2} D_{3 / 2} - 5 f^{2} F_{5 / 2}^{°}$
21	9 746.726	10 257.04	$7 d^{2} D_{5 / 2} - 6 p^{2} P_{3 / 2}^{°}$
16	10 019.461	9 977.84	$7 d^{2} D_{3 / 2} - 6 p^{2} P_{1 / 2}^{°}$
1	10 603.776	9 428.02	$9 s^{2} S_{1 / 2} - 6 p^{2} P_{3 / 2}^{°}$
2	19 669.104	9 370.29	$5 d^{2} D_{5 / 2} - 6 f^{2} F_{7 / 2}^{°}$
2	10 692.451	9 349.83	$5 d^{2} D_{3 / 2} - 6 f^{2} F_{5 / 2}^{°}$
1	10 902.049	9 170.07	$9 s^{2} S_{1 / 2} - 6 p^{2} P_{1 / 2}^{°}$
1	11 220.686	8 909.66	$8 d^{2} D_{3 / 2} - 6 p^{2} P_{3 / 2}^{°}$
1	11 239.857	8 894.47	$8 d^{2} D_{5 / 2} - 6 p^{2} P_{3 / 2}^{°}$
1	11 490.7	8 700.30	$5 d^{2} D_{5 / 2} - 7 f^{2} F_{7 / 2}^{°}$
1	11 514.0	8 682.69	$5 d^{2} D_{3 / 2} - 7 f^{2} F_{5 / 2}^{°}$
1	11 518.956	8 678.96	$8 d^{2} D_{3 / 2} - 6 p^{2} P_{1 / 2}^{°}$

Designation	This Paper	Ref. 1	Ref. 25
Odd Configurations
$5 s^{2} (^{1} S) 6 p^{2} P_{1 / 2}^{°}$	31 816.982	31 816.61	31 816.96
${{}^{2}P}_{3 / 2}^{°}$	32 115.251	32 114.79	32 115.22
$5 s^{2} (^{1} S) 7 p^{2} P_{1 / 2}^{°}$	38 861.448	38 861.35	38 861.43
${{}^{2}P}_{3 / 2}^{°}$	38 972.911	38 972.84	38 972.90
$5 s^{2} (^{1} S) 4 f^{2} F_{5 / 2}^{°}$	39 707.161	39 707.29	39 707.59
$F_{7 / 2}^{°}$	39 707.622	39 707.96
$5 s^{2} (^{1} S) 8 p^{2} P_{1 / 2}^{°}$	41 827.167	41 827.10
$5 s^{2} (^{1} S) 8 p^{2} P_{3 / 2}^{°}$	41 881.457	41 881.44
$5 s^{2} (^{1} S) 5 f^{2} F_{5 / 2, 7 / 2}^{°}$	42 220.281	42 220.0	42 220.25
$5 s^{2} (^{1} S) 6 f^{2} F_{5 / 2, 7 / 2}^{°}$	43 584.681	43 584.4	43 584.66
$5 s^{2} (^{1} S) 7 f^{2} F_{5 / 2, 7 / 2}^{°}$	44 406.23	44 406.20(5/2)	44 406.31
		44 406.26(7/2)
$5 s^{2} (^{1} S) 8 f^{2} F_{5 / 2, 7 / 2}^{°}$	44 938.845	44 938.71(5/2)	44 938.81
		44 938.70(7/2)
Even Configurations
5s²(¹S)6s²S_1/2	24 372.956	24 372.87	24 372.956
5s²(¹S)5d²D_3/2	32 892.230	32 892.12	32 892.21
²D_5/2	32 915.539	32 915.42	32 915.54
5s²5p^{2 4}P_3/2	36 020.519	36 020.80
⁴P_5/2	37 451.970	37 451.90
5s²(¹S)7s²S_1/2	36 301.864	36 301.69	36 301.84
5s²(¹S)6d²D_3/2	39 048.576	39 048.48	39 048.53
²D_5/2	39 098.464	39 098.37	39 098.38
5s²(¹S)8s²S_1/2	40 636.996	40 636.71	40 636.98
5s²(¹S)7d²D_3/2	41 836.443	41 836.23	41 836.41
²D_5/2	41 861.978	41 861.57	41 861.96
5s²(¹S)9S²S_1/2	42 719.031	42 718.55	42 719.02
5s²(¹S)8d²D_3/2	43 335.937	43 335.63	43 335.93
²D_5/2	43 355.108	43 354.62	43 354.08
5s²(¹S)10S²S_1/2	43 881.314	43 880.83	43 880.26
5s²(¹S)9d²D_3/2	44 234.704	44 234.26	44 234.70
²D_5/2	44 249.829	44 249.37	44 249.77
5s²(¹S)11S²S_1/2	44 596.443	44 595.86
5s²(¹S)10d²D_5/2	44 827.475	44 827.02

Abstract

Cited By

Figures (2)

Tables (3)

Equations (74)

Journal of the Optical Society of America B