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High-order stimulated Raman scattering in a highly transient regime driven by a pair of ultrashort pulses

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Abstract

We demonstrate efficient generation of high-order anti-Stokes Raman sidebands in a highly transient regime, using a pair of 100-fs laser pulses tuned to Raman resonance with vibrational transitions in methane or hydrogen. The use of this technique looks promising for efficient subfemtosecond pulse generation.

© 2004 Optical Society of America

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