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Dispersion of the resonant nonlinear optical susceptibility obtained with femtosecond time-domain coherent anti-Stokes Raman scattering

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Abstract

We propose and experimentally demonstrate a method that is capable of resolving both real and imaginary parts of third-order nonlinearity (χ(3)) in the vicinity of Raman resonances. Dispersion of χ(3) can be obtained from a medium probed within microscopic volumes with a spectral resolution of better than 0.10cm1.

© 2013 Optical Society of America

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