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Development of a combined pure rotational and vibrational coherent anti-Stokes Raman scattering system

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Abstract

A combined pure rotational coherent anti-Stokes Raman scattering (PRCARS) and vibrational CARS (VCARS) system has been developed. In this system two beams, a broadband beam centered at 607 nm and the frequency-doubled Nd:YAG output at 532 nm is used to generate the PRCARS signal. A second 532 nm beam is used along with the other two beams to simultaneously generate the N2 VCARS signal using a standard phase-matching scheme.

© 2013 Optical Society of America

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