Abstract
In this paper, we demonstrated an active dual tunable broadband terahertz absorber with polarization-independent characteristic, which consists of a hybrid graphene-vanadium dioxide (VO2) metasurface array and a VO2 ground plane separated by a dielectric layer. Numerical simulation results indicate that there are the most distinctive broad absorption spectra and a bandwidth with an absorptance over 90% as wide as 1.7 THz. Blue shift occur in the perfect absorption peaks of the absorber, which shift 1.18 THz from 0.1 eV to 0.6 eV by adjusting the Fermi energy of graphene. Additionally, by using external stimuli to change the conductivity of the VO2, the corresponding absorptance can be continuously adjusted from 28% to 99%, indicating that we can modulate the amplitude on the absorption spectrum. Therefore, we can achieve the tunable property in both frequency and amplitude through an external stimulus on the proposed simple structure. The electric field distribution and impedance matching theory can be explained the inherent physical mechanism. The absorber is effective to reach a 0°∼75° range of incident angles for both TE and TM polarizations. It indicates that the proposed absorber is beneficial to a new design method for high-performance terahertz devices.
© 2020 Optical Society of America under the terms of the OSA Open Access Publishing Agreement
1. Introduction
Metamaterial functional device, is an artificially engineered periodic nanostructure with the subwavelength scale unit cell. In the past decade, many researchers have been devoted to filling the “THz gap” due to great potential applications of THz functional devices [1–3]. Since then, THz functional devices have become one of the most attractive aspects of research in the modulator, biological imaging, spectroscopy, and so on [4–7]. Among all the applications, various kinds of absorbers are reported to achieve excellent absorption performance consists of single-band [8–9], multi-band [10–11], and broadband [12–14] since the perfect absorption theory is firstly proposed by Landy et al., in 2008 [8]. However, it is not easy for these traditional structures to change the working bandwidth and absorption intensity when the non-tunable materials are used. So, the tunable metamaterial absorbers emerge at a historic moment, it is a frequency (amplitude) modulator whose absorption performance can be adjusted by applying external stimuli [14–17]. One experimentally demonstrated pathway to achieve tunable property is to apply tunable materials to design, such as graphene [14–15], phase-change materials (PCMs) [16–17], and liquid crystal [11].
Among various tunable device in the THz range, graphene- or vanadium dioxide (VO2)-based broadband metamaterial absorbers have attracted remarkable attention due to their active tunable (switchable), unique electromagnetic, and optical properties [18–22]. Huang et al., proposed a classical sandwich broadband THz absorber based on graphene, and the peak absorption can be tuned from 19% to 100% by changing the Fermi energy of graphene [23]. Zhang et al., designed a tunable and broadband metamaterial absorber in the mid-infrared region based on hybrid graphene-gold metasurface, and with the increase of graphene's Fermi energy, the resonance frequency of the absorber blue shifts [14]. Liu et al., reported a broadband tunable metamaterial absorber, based on the unique transition character of VO2, the maximum tunable range of the proposed absorber can be realized from 5% to 100% by an external thermal excitation [24]. Furthermore, by applying both graphene and VO2 materials in a simple sandwich structure, the tunable performance of the device can be further improved. Wang et al., propose a dual-controlled switchable broadband terahertz absorber based on a hybrid of VO2 and graphene, using these two independent controls in tandem, it found that the state of the proposed absorber can be switched from absorption to reflection [18]. Zhang et al., proposed a terahertz bifunctional absorber is presented with broadband and narrowband absorbing properties based on hybrid graphene-VO2 metamaterial [19]. Previous studies indicate that both graphene and VO2 materials can be used to design tunable terahertz metamaterial functional devices. But so far, there is no simple sandwich structure that can simultaneously achieve the characteristics of tunable in both absorption intensity and frequency, which is a huge challenge for researchers.
In this paper, we proposed an exquisite polarization-insensitive broadband terahertz absorber that can achieve an active tunable property in both magnitude and frequency on a simple sandwich structure. Consists of the perfect absorption peaks of the device can be tuned by adjusting the Fermi energy of graphene, which blue-shift 1.18 THz from 0.1 eV to 0.6 eV. By using external stimuli to change the conductivity of the VO2, the absorptance of the corresponding absorption spectrum can be continuously adjusted from 28% to 99%. An excellent absorption performance over a wide range of incident angles up to 70° in the terahertz regime. It indicates that the proposed structure is beneficial to a new design method for high-performance terahertz devices.
Indeed, our results are better indicated in the recent work based on dual-control systems, both Ref. [18] and Ref. [25] have studied the polarization-dependent sandwich structure with dual-control characteristics at the THz range. When it is in the perfect broadband absorption state, the amplitude (perfect absorption peaks) of the absorption spectrum can be tuned by changing the chemical potential of graphene (Dirac semimetal) or the conductivity of VO2. Although these works presented dual-control of the absorptance, however, our designed simple structure achieves a widened range of dynamically tunable property in both of amplitude and frequency in the THz range, simultaneously. Meanwhile, the absorber of our report shows the strong incident angle insensitive property and indicates practical operability.
2. Structure and methods
The schematic of the proposed broadband absorber based on hybrid graphene-VO2 metamaterials is given in Fig. 1. The absorber is composed of a symmetric E-shaped resonator array on top of a continuous monolayer graphene sheet, which is supported by a dielectric spacer backed with a reflective mirror. At the designed system, unlike most traditional metamaterial absorbers, both of the symmetric C-shaped resonator array and bottom reflective film use a common phase change material of VO2. By controlling the insulator-to-metal transition (IMT) of VO2, we can achieve the proposed structure to function as a unity-broadband THz metamaterial absorber. Besides, both of the thickness of the top VO2 resonator array and ground plane are optimized as $t = 0.3\; \mu m$, it can be easily manufactured by molecular beam epitaxy in practical application [26,27]. Here, the dielectric spacer is defined as ToPaS with a complex electric permittivity ${\varepsilon _s} = 2.35\, + \,0.01i$ [23] and a thickness of ${t_s} = 20\; \mu m$. The structural dimensions of the proposed absorber are listed as follows: $P = 50\; \mu m,\; {t_1} = 2\; \mu m,\; L = 30\; \mu m,\; G = 5\; \mu m,$ and $W = 2\; \mu m$.
Indeed, VO2 has been studied for different applications based on its metal-insulator phase transition at ∼68°C [27]. Since metallic VO2 has a high free carrier concentration, it can achieve a significant modulation depth in application [28]. Moreover, in the insulated state, it is highly transparent to electromagnetic waves below 6.7 THz [29]. The optical properties of VO2 in the THz range can be modeled by the Drude model [18–21]
In addition, the monolayer CVD graphene is molded as an equivalent 2D surface impedance layer and without thickness [26,30]. From the range of terahertz to optical frequency, the graphene’s surface conductivity ${\sigma _g}(\omega )$ can be described as ${\sigma _g}(\omega )= {\sigma _{inter}}(\omega )+ {\sigma _{intra}}(\omega )$, which consists of intra-band ${\sigma _{intra}}(\omega )$ and inter-band ${\sigma _{inter}}(\omega )$ contributions from the Kubo formula, respectively. However, according to the Pauli exclusion principle, the inter-band contribution is negligible compared to the intra-band part as the photon energy $\hbar \omega \ll {E_f}$ and ${k_B}T \ll {E_f}$ in the THz range [23]. Therefore, the surface conductivity of graphene can be simplified to ${\sigma _g}(\omega )= {\sigma _{intra}}(\omega )$ and the intra-band ${\sigma _{intra}}(\omega )$ can be defined as [31–32]:
3. Results and discussions
When the Fermi energy of graphene is set to 0.1 eV and the VO2 was in a fully metallic state with conductivity of 200000 S/m, the designed system can realize broadband absorption. The absorption, reflection and transmission spectrums for the transverse-electric (TE) polarization under normal incidence are given in Fig. 1(a). There is most distinctive broad absorption spectrum, and the bandwidth with absorptance over 90% are starting from 1.7 THz to 3.4 THz. Also, it can be found that there are also two near-unity absorption peaks located at ${f_1}$=2.3 THz and ${f_2}$=3.2 THz, respectively. To further reveal the working mechanism for the proposed device, the impedance matching theory is introduced. Therefore, the absorptance and the relative impedance can be defined as [35,36]:
To better grasp the absorption mechanism in the whole broadband absorption spectrum, as shown in Fig. 3, we monitor the electric field distribution for different resonance frequencies. It can be seen that the absorptance at 0.1 THz is only 1%, it means that there is almost no electric field distribution of the device, indicating that the absorber does not interact with the incident waves. As shown in Fig. 3(a), when the frequency shift to 0.6 THz, the corresponding absorptance is varied to about 18%. It seems like a weak resonant response is generated in the symmetric C-shaped metasurface and the electric field is coupled at both corners of the arms. Next, we have monitored the electric field distributions at the strong resonance frequencies of 1.5 THz, and 2.3 THz with the absorptance above 80%, respectively. From Figs. 3(a) and 3(b), the electric energy is strongly concentrated on the whole surface of the symmetric C-shaped array, and a strong electric energy is concentrated on the interface between the dielectric and the graphene sheet. It means that the graphene surface plasmon resonances (SPR) can also enhance the absorption performance. In contrast, when the resonance frequency shifts to 3.2 THz and 3.7 THz, the coupled electric field intensity is gradually reduced, as shown in Fig. 3(a), we can obtain that the resonant response gradually disappears and the absorptance decreased. Indeed, it can be seen from Fig. 3(b) that the local magnetic resonance is caused by the coupling between the adjacent unit lattice and the metal phase grounding plane so that the electric field distribution presents a typical high-order mode. From the side view of the absorber, as the frequency increases, it can be seen that the inside electric field distribution has a tendency to strengthen. However, the power loss of electromagnetic energy in the top graphene layer gradually increases with the increasing frequency according to Ref. [14], so the absorptance will decline.
The surface conductivity of the graphene sheet layer can be dynamically tuned by varying its Fermi energy from 0.1 eV to 0.6 eV, thus leading to a blue-shift on the absorption spectra. The resultant frequency shift can be defined as [14,37]
Next, Fig. 5(c) depict the absorption spectrums of the proposed absorber with different conductivities of VO2 at perfect absorption of 2.3 THz when the Fermi energy of graphene is set to 0.1 eV. It is clear that with the conductivity of VO2 increases from 10 S/m to 200000 S/m, the corresponding absorptance dynamically adjusted from 28% to 99% for the broad absorption band of 1.7 THz to 3.4 THz. It means that we can continuously modulate the amplitude on the absorption spectrum. On the other hand, as shown in Figs. 5(d) and 5(e), according to the side view of the electric field distributions, When the VO2 is in the metallic state, a strong electric field is mainly concentrated on the interface between the dielectric spacer and the hybrid metasurface. It indicates that the graphene plasmon resonances can enhance the absorption performance, while the electric field distributions are quickly decreased to zero when VO2 is in the insulating state. Furthermore, the variation of permittivity of VO2 mainly decides the relevant physical mechanism of the continuous modulation of amplitude. Specifically, we can see that the real parts under different conductivities of VO2 are much smaller and almost unchanged than that of imaginary parts, as the Figs. 5(a) and 5(b) shows, the real and imaginary parts of the permittivity of VO2. It means that the real parts of the permittivity mainly decide the resonance frequency; however, the imaginary parts mainly decide the loss of amplitude. Therefore, the positions of two broad bands almost unchanged, while the intensity of the absorption spectra varies significantly from the proposed absorber.
When we changed the conductivity of VO2 in both top and bottom layers simultaneously, we introduced the impedance matching theory to clarify the internal mechanism. As shown in Fig. 6, the real and imaginary parts of the relative impedance ${Z_r}$ under different conductivity of VO2. One can clearly see that the real part gradually approaches to 1, while the imaginary part gradually approaches to 0 with the dynamically increase conductivity of VO2, in the broadband frequency range of 1.7 THz to 3.4 THz. It means that the impedance between the proposed absorber and the free space gradually matches when the IMT properties occurs from VO2 of the bottom layer. Therefore, a high modulating intensity is obtained.
To demonstrate the absorptance of the absorber can achieve an active tunability of wide range with the control of the special VO2 phase change material. From Figs. 7(a)–7(f), we further monitor the electric field distribution for the heating process with different conductivity of the VO2 at the perfect absorption of 2.3 THz. It can be seen that there is almost no electric field distribution of the symmetric C-shaped array at the conductivity $\sigma ({V{O_2} = 10\; S/m} )$. It means that the incident THz waves completely penetrate the proposed structure due to the insulation properties of VO2. Therefore, one can clearly see that as the VO2 material is gradually transformed from the insulation-phase to full metal-phase under normal incidence, the electric field distributions are mainly concentrated on the concerns of the symmetric C-shaped VO2 arms and gradually diffused to the whole and the cross area of the arm, when the conductivity of VO2 raise from 100 S/m to 200000 S/m. The reflection of the symmetric C-shaped resonant structure and the metal-phase VO2 reflective plane are enhanced synchronously, which causes an intense increase in the absorptance. Besides, it can be seen that the electric field distributions are almost the same in both $\sigma ({V{O_2} = 40000\; S/m} )$ and $\sigma ({V{O_2} = 200000\; S/m} )$. Due to the VO2 material is completely transformed into its metal-phase, thus the resonant induced by the symmetric C-shaped VO2 structure will not be further changed with the increasing conductivity. Therefore, the proposed structure can achieve the alternation between the full transmission and the broadband absorption in the THz region based on external stimuli.
To further evaluate the importance geometrical parameters of the effect on performance, we also investigated the absorption spectra with different geometric parameters under normal incidence, keeping other structural parameters unchanged of the unit cell. As shown in Fig. 8(a), where the influence of the absorptance on the width W is simulated. One can clearly see that with the increasing width W from 2 μm to 14 μm, the broad absorption spectra is disappeared and gradually splits into two narrow bands. As shown in Fig. 8(b), The influence of the length of arm L on absorption performance is also investigated. It can be seen that the absorption spectrum is broadened gradually and the absorptance is also enhanced when the arm length changing from 20 μm to 30 μm. The symmetric C-shaped resonant properties are mainly thanks to the electric field coupled to the arms. On the other hand, it can be explained by the impedance matching theory. The excellent impedance matching between the absorber and free space is broken with the arm length decreasing. Besides, as shown in Fig. 8(c), it can be seen that the absorption curves of different gap width are perfectly coincident. To better understand the physical mechanism of the absorption spectrum, the results of analyzing the electric field distributions of the gap width of G fixed at 2 μm, 5 μm, and 8 μm, respectively at the resonance frequency of 2.3 THz are displayed in Fig. 8(d). Although the gap width of G has changed, the graphene surface plasmon resonance is stably excited, which is the key to keep the absorption performance stable. Therefore, this may have great operability in practical applications.
When VO2 is in the metallic state, it is indispensable to explain the main contribution to THz absorption performance of each part in the designed sandwich structure. So, the influences of dielectric loss (tagδ=0.1) in the middle spacer on absorption performance are investigated. As we can see from Fig. 9(a), it confirms that there is no evident change in the broad absorption spectrum, the dielectrics have a limited influence on the THz absorption. The insensitivity of dielectric spacers in the proposed absorber can be property applicable in many areas due to the existence deviation in practical fabricate, such as tunable modulators [36]. As shown in Fig. 9(b), one can clearly see that the achieved maximum absorption without VO2 film dielectric in the corresponding spectrum is only 28%, much smaller than that with the VO2 plane. Besides, from Fig. 9(c), absorbers based on the single C-shaped resonator are also studied. It can be seen that the two broad absorption bands are perfectly coincident due to the symmetry of the proposed device. In addition, although both of the two absorbers based on a single C-shaped resonator exhibit limited absorptance and the narrow spectrum bandwidth. However, it can be seen that absorbers based on the symmetric C-shaped can enhance the resonant and lead to strong broad absorption. Indeed, we purposely utilize the coupling effect between the two C-shaped resonant to achieve the excellent performance of the absorber. Then, we consider the effect of the proposed absorber with and without symmetric C-shaped VO2 resonant structures on the absorption performance. We found that the addition of the symmetric C-shaped resonance structure on the proposed absorber can enhance the absorptance and effectively expands the impedance matching bandwidth from the Fig. 9(d). Thus, based on the previous analysis, it can be confirmed that the energy of incident THz waves is mainly concentrated on the hybrid symmetric C-shaped VO2 resonance metasurface.
As shown in Fig. 10(a), it is obvious that the absorption curves under different polarization angles have completely coincided when the bottom layer in metal-phase, which indicates that the proposed absorber could work well with different polarization modes. Indeed, the symmetric unit cell is the inherent reason for the perfect polarization-independent. On the other hand, the incident electric energy is stably excited, which is the key to keep the absorptance stable are displayed in Figs. 10(b)–10(e).
The influences of different incident angles on the absorption performance in both the TE and TM modes are also investigated in Fig. 11. For TE polarization, the broad absorption band exhibit excellent absorption performance with incidence angles vary from 0° to 80°. The absorption peaks remain more than 80% until the incident angle exceeds 70°. It is found that the absorption frequency range is almost constant as the incident angle increases for the absorption spectrum and some parasitic resonances that occurred at the larger incident angle from the Fig. 11(a) [18]. For TM polarization, the results are similar to TE mode apart from that the absorption peaks split to two for large incidence angles and there is a slightly blue-shift for the absorption spectrum are displayed in Fig. 11(b). In addition, both of the two absorptances peaks decrease significantly as the incident angle is further increased up to 75°. On the other hand, the propagation constant ${k_z}$ along z-direction is molded by ${k_z} = {k_p}({1 - si{n^2}\xi } )$ [38,39], where ${k_p}$ is the wave number in dielectric layer. We can find that the phase-matching condition is not satisfied on the graphene surface since ${k_z}$ increases with the incident angel, it means that the excellent impedance matching is destroyed, which will weaken the absorption performance for the proposed absorber.
4. Conclusion
In the conclusion, we proposed and demonstrated an active tunable broadband metamaterial absorber based on hybrid graphene-vanadium dioxide, polarization-insensitive properties are achieved in the absorber. The broadband absorption of the absorber maintains excellent absorption performance over a wide range of incident angles up to 80°. Apparently, by applying an external bias voltage to adjust the Fermi energy of graphene, the perfect absorption peaks frequency of the absorber occurs blue shifts, which shift 1.18 THz from 0.1 eV to 0.6 eV. Numerical simulation results indicate that the absorptance of the proposed absorber can be dynamically adjusted from 28% to 99% for the broad absorption band of 1.7 THz to 3.4 THz by adjusting the conductivity of the VO2 due to its unique IMT properties. The impedance matching theory is introduced to explain the inherent physical mechanism. Thus, we can achieve the tunable property in both frequency and amplitude through an external stimulus on a simple structure. Following the electric field distribution can explain the absorption mechanism of the absorber. Therefore, we present a new design method for high-performance terahertz devices.
Funding
National Natural Science Foundation of China (61162004).
Acknowledgments
Thanks, due to Wenhui Xu for valuable discussion.
Disclosures
The authors declare no conflicts of interest.
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