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Omnidirectional constant transmission and negative Brewster angle at planar interfaces associated with a uniaxial medium

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Abstract

This paper presents our detailedly theoretical analyses on omnidirectional constant transmission and negative Brewster angle at planar interfaces associated with a uniaxial medium. The amplitude reflection and transmission coefficients at planar interfaces associated with uniaxial media are derived by examining the boundary condition and the dispersion relation. It is found that under certain conditions, the coefficients are constants independent of the incident angle. Another interesting phenomenon is that an interface between isotropic and uniaxial media can exhibit negative refraction under Brewster condition. Our results offer considerable potential device applications of uniaxial media.

©2009 Optical Society of America

1. Introduction

The phenomena of reflection and refraction of light at the interface of two transparent media are widely used for controlling the intensity, phase, polarization and direction of light in many optical devices [1]. Such phenomena in anisotropic media may be much different from those in isotropic media thus have recently attracted increasing amount of attention [211]. Negative refraction, which was of great interests these years [1214], can be induced by anisotropy [25] under sufficiently small incidence. It is well known that the amplitude reflection and transmission coefficients [15] at a planar interface of two isotropic media depend on the incident angle. And the refraction requires refractive index mismatch, which seems to inevitably result in a finite reflection loss except at particular oblique incidence like Brewster angle. However, it is not always true for the case of a planar interface associated with a uniaxial medium. Recent experiment [6] demonstrated a very interesting phenomenon, omnidirectional total transmission, which means that the wave is totally transmitted for arbitrary incoming direction at a unique type of the interface of twinning structures using uniaxial crystals. The phenomenon can also occur at interface between isotropic and uniaxial media [7] by appropriate refractive index matching and optical arrangement of the optical axis of a uniaxial medium. Another property in anisotropic system is that the Brewster angle can be tuned from 0° to 90° under certain conditions, which is much different from in isotropic case [810]. Abnormal total reflection can also occur in anisotropic media [11]. However, all these properties can be derived by investigating the amplitude reflection and transmission coefficients. In this paper, we show theoretically that omnidirectional constant transmission is available at planar interfaces associated with a uniaxial medium. In addition, although negative refraction caused by anisotropy can only occur for small incident angle, it may occur without reflection loss under Brewster condition.

2. Theory

The incident wave is assumed to be a monochromatic uniform electromagnetic (EM) plane wave with an optical frequency ω and a space-time dependence specified by exp(i k·r-iωt) which has been omitted in the following as for simplification. As shown in Fig. 1 , the relation between the principal axes of the anisotropic medium (x,y,z) and the surface coordinates (x,y,z) can be expressed as

x=xcosθ+z'sinθ,y=y,z=xsinθ+z'cosθ,
where θ is the inclined angle of the optical axis to the surface. Since the media are isotropic in the y–z plane, the wave vectors can be assumed to be in the x–z plane without losing any generality. In this section we will only examine the case of incidence from the uniaxial medium 2, and medium 1 is isotropic.

 figure: Fig. 1

Fig. 1 Principal axes of the anisotropic medium (x,y,z) and the surface coordinates (x,y,z).

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In a uniaxial medium, when extraordinary TM waves (Ey = Hx = Hz = 0) are of interest, in the principal axes’ coordinates, the EM field can be expressed as

H=(0,H0,0),E=(kzH0/ωε0εx,0,kxH0/ωε0εz),
and the wave vector components kx and kz satisfy the following dispersion relation:
kx2/εz+kz2/εx=k02,
where kx and kz are, the x and z components of the wave vectors respectively, and k 0=ω/c with c is the speed of light in vacuum.

The wave vector components of the incident, the reflected and the transmitted rays parallel to the interface must satisfy the boundary condition:

kix'=krx'=ktx'B,
where the subscripts i, r and t denote the incident, reflected and transmitted ray respectively, and the superscript “” denotes the surface coordinates. For isotropic medium 1 with refractive index nt, B can be deduced from B = ntsinθt k 0, where θt is the refractive angle.

From Eq. (1), the dispersion relation in the surface coordinates becomes:

αB2+βBkz'+γkz'2=k02εzεx,
where
α=εxcos2θ+εzsin2θ,β=(εxεz)sin2θ,γ=εxsin2θ+εzcos2θ.
Solutions of kz in Eq. (5) are
kz±'=βB/2γ±A
with
A=[εzεx(γk02B2)]1/2/γ.
Both kiz and krz satisfy Eq. (5). To take simplify but without lose of generality, we set kiz = kz- and krz = kz+ on the following.

It is easy to get the expressions of the EM wave in the surface coordinates:

H=(0,H0,0),E=(γkz'+βB/2,0,αBβkz'/2)H0/ωε0εzεx.
The amplitude reflection coefficient r and transmission coefficient t can be obtained using the boundary condition. From Eqs. (7) and (9), the incident and reflected EM waves can be written as
Hi=(0,H0,0),Ei=(γA,0,αBβkiz'/2)H0/ωε0εzεx
and
Hr=r(0,H0,0),Er=r(γA,0,αBβkrz'/2)H0/ωε0εzεx
separately. Assuming medium 1 is isotropic with permittivity ε 0 ε 1, the corresponding transmitted EM waves is expressed as
Ht=t(0,H0,0),Et=t(ktz',0,B)H0/ωε0ε1.
The EM waves components parallel to the interface must be continuous to satisfy the boundary condition, so the amplitude reflection and transmission coefficients can be deduced as
r=Hr/Hi=(γA/εzεxktz/ε1)/(γA/εzεx+ktz/ε1),
t=Ht/Hi=(2γA/εzεx)/(γA/εzεx+ktz/ε1).
From Eq. (9), the time-averaged Poynting vector in the surface coordinates is given as
S=Re[(αB+βkz'/2,0,γkz'+βB/2)H02/2ωε0εzεx].
Using Eqs. (7) and (15), the incident and reflected angles of ray vectors can be proved to be

tgθsi=Six'/Siz'=β/2γ+Bεxεz/Aγ2,
tgθsr=Srx'/Srz'=β/2γ+Bεxεz/Aγ2.

3. Results and discussions

For the case of incidence from the uniaxial medium, comparing with the isotropic cases, it can easily find that kiz/εi is replaced by γA/εzεx in the amplitude reflection and transmission coefficients. In a similar way, the coefficients can be easy written down by same replacements in cases of wave incident from the isotropic medium and at an interface of two uniaxial media. For a fixed incident angle, the coefficients can be tuned by γ with changing θ, which gives a new way to control the amplitudes of reflected and transmitted waves as well as the Brewster angle.

It should be noted that omnidirectional total transmission has been discussed in Ref [6, 7]. without presenting the amplitude reflection and transmission coefficients. From Eq. (13) it can easy be seen that omnidirectional total transmission occurs at the surface between a uniaxial medium and an isotropic medium under condition of γA/εzεx = ktz/ε 1, which means

γ=ε1
and
εzεx=ε12.
Equations (13) and (14) also show that under condition of γ=(εzεx)1/2, the coefficients have the same forms as isotropic media on both sides with refractive indexes (εzεx)1/2 and ε 1. So with a proper θ giving γ=(εzεx)1/2, a uniaxial medium can be considered as an equivalent isotropic medium of εeq=(εzεx)1/2 in some means. If εeq 1, omnidirectional total transmission yields at the interface as if the same media on both sides, which is the essence of omnidirectional total transmission in this case. However, refraction is still in existence for the directions of wave vector and ray vector change after transmission in most of the cases. For uniaxial media on both sides, omnidirectional total transmission can happen when γ 1 A 1/εz 1 εx 1=γ 2 A 2/εz 2 εx 2, which means γ 1=γ 2 and εz 1 εx 1 = εz 2 εx 2. From Eq. (6) one can immediately conclude that θ 2= 1 at the surface between the same uniaxial media with arbitrary θ 1, omnidirectional total transmission occurs.

From above discussion, both Eqs. (17a) and (17b) must be fulfilled for omnidirectional total transmission. A question arised naturally is what happens if only one of the equations is fulfilled. From Eq. (14), the condition for omnidirectional constant transmission (amplitude transmission coefficient is a constant irrespective of the value of B) is Eq. (17a), which gives match of wave vectors so that the amplitude reflection and transmission coefficients keep constantly in spite of the variation of the incident angle. In addition, Eq. (17b) can be considered as giving match of refractive index so that reflected wave disappears and omnidirectional total transmission occurs under condition of wave vectors matching.

When ε 1 is between εz and εx, θ can be chosen to be ±arcsin[(ε 1 z)/(εxz)]1/2 to fulfill Eq. (17)a), and the amplitude reflection coefficient is a constant for arbitrary incident angle:

r=[1/(εzεx)1/21/ε1]/[1/(εzεx)1/2+1/ε1].
It is obvious that omnidirectional total transmission, where both Eqs. (17a) and (17b) are fulfilled and r=0, is a special case of omnidirectional constant transmission. However, the condition for omnidirectional constant transmission is much looser than for omnidirectional total transmission and is easy to meet. At the wavelength of 632.8 nm, if using calcite as the uniaxial medium with ε x=1.4862 and εz=1.6582 one can find there are a lot of isotropic media with ε 1 between ε z and ε x, e.g. Ba(NO3)2, CdF2, CsCl and NaCl, which can be chosen [16] to realize omnidirectional constant transmission but not omnidirectional total transmission.

It should be pointed out that the amplitude reflection and transmission coefficients are still constants even at incident angle of near 90° and total reflection never occurs under condition of Eq. (17a). Otherwise, total reflection may occur at graze incidence from one side. For γε 1, the amplitude reflection coefficient changes dramatically near the critical angle. For example, if the incident angle θ of the 632.8 nm beam is 84° from isotropic side, and calcite is used in the other side, the refractive index of an isotropic medium changes from γ 1/2 to γ 1/2+0.01, absolute value of the amplitude reflection coefficient can change from 0.0011 to 1. Such property can be used for a filter with highly sensitive intensity control and a new kind of optical bistable switch. However, the mechanism and an easy way to change the refractive index still need to be found out.

The discussion above shows that the amplitude reflection and transmission coefficients can be constant. However, for a beam splitter the reflectivity and transmissivity [1] (the ratios of power) are of much interest. From Eqs. (10) and (11), it can be shown that

Si=Re[(αB+βkiz'/2,0,γA)H02/2ωε0εzεx],
Sr=Re[(αB+βkrz'/2,0,γA)r2H02/2ωε0εzεx].
The intensities of incident and reflected wave are Ii = S’i and Ir = S’r. It is easy to prove that Ii/Ir is not equal to ׀r׀2 but has a more complex expression since kizkrz in Eqs. (19) and (20) because the reflected angle is not equal to the incident angle in most of the case in an anisotropic medium and the cross section of the wave changes after reflection. So constant transmission of amplitude indicates constant transmission of power is not straight forward for anisotropic case. Here we further examine how the incident field is divided into the reflected and transmitted fields and calculate the reflectivity and transmissivity. The amount of energy in the incident wave on a unit area of the boundary per second is therefore Ji=S’icosθsi=S’iS’iz/S’i=S’iz, and the energy of the reflected wave leaving a unit area of the boundary per second is given by similar expressions Jr = -S’rz. So using Eqs. (19) and (20), the reflectivity can be given as
R=Jr/Ji=|r|2.
And the transmissivity can be given as
T=1|r|2
from energy conservation. Equations (21) and (22) indicate that omnidirectional constant transmission gives a result of omnidirectional constant reflectivity and transmissivity. Such property can be used for a beam splitter with splitting ratios independent with incident angle. It is quite useful for a beam splitter as well as an attenuator under wide incidence. What is more, the adjusting precision can be greatly reduced with great improvement of insensitivity on excursion. For a fixed anisotropic medium, such beam splitter can be designed by choosing isotropic media with refractive indexes between εx 1/2 and εz 1/2 and rearrange the optical axis to tune the omnidirectional constant reflectivity from 0 to (εx 1/2 z 1/2)2/(εx 1/2 z 1/2)2, which is from 0 to 0.003 for calcite crystal.

Now we turn our attention to the Brewster angle. The definition of Brewster angle can be extended to the surfaces of transparent uniaxial crystals [9]. In isotropic cases, the Brewster angles are given as tanθB 1 =n 2/n 1 and tanθB 2 =n 1/n 2 with θB 1 and θB 2 are the Brewster angles of medium 1 (with refractive index n 1) and medium 2 (with refractive index n 2) at an interface between them. In optically anisotropic surfaces, from Eq. (13), the expression of B for r=0 is

B2=(εxεzε1γ)ε1k02/(εxεzε12),
and the Brewster angle θB 1 is given by
tan2θB1=(εxεzε1γ)/(ε1γε12).
So the existence and size of θB 1 depend on γ for fixed εx, εz, and ε 1. Brewster angle exists under condition that γ is between ε 1 and εxεz/ε 1. For ε 1 is between εx and εz, θB 1 can be tuned from 0 to 90° by changing γ [9]. It should be pointed out that under condition of Eq. (17a) θB 1 is equal to 90° and loses its meaning. However, the numerator and the denominator of the right side of Eq. (24) are both 0 under conditions of Eqs. (17a) and (17b). So θB 1 can be considered as uncertain when omnidirectional total transmission happens.

We can get the relation of θB 1 and θB 2 from Eqs. (16), (23) and (24):

tan2θB1/(tanθB2±±|β|/2γ)2=ε12/γ2.
So for Brewster angle θB 1 of isotropic medium 1, there are two Brewster angles of anisotropic medium 2. The smaller angle θB 2+ corresponding to “+” and the larger angle θB 2- corresponding to “_” in Eq. (25), which are different for wave propagating from right to left or the inverse. Under the condition γεxεz/ε 1, Brewster angle θB 1 can be sufficiently small so that θB 2+ is negative thus negative refraction happens under Brewster condition. From Eqs. (24) and (25), numerical calculation shows that the Brewster angle θB 2+ can be negative while θB 1 is between 0 and 6.1°. When γε 1, all the Brewster angles are near 90°. The relations of Brewster angles and γ at the surface of Ba(NO3)2 (ε 1=1.57142) and calcite are shown in Fig. 2(a) with γ changing from εxεz/ε 1 to ε 1. The Brewster angles are sensitive in dependence on γ as well as refractive indexes thus may provide a new technique for optical axis orientation and refractive indexes measurement. A frequency-selective device may also be derived by selecting a dispersive uniaxial medium such that Brewster angles are different for different frequencies.

 figure: Fig. 2

Fig. 2 (a)Brewster angles θB 1 and θB as functions of γ at the surface of Ba(NO3)2 (ε 1=1.57142) and calcite (εx=1.4862, εz=1.6582); (b)Brewster angle θB 1 and critical angle θc 1 as functions of γ at the same kind of surface.

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If γ<ε 1, total reflection can occur for wave incident from medium 1, and the corresponding critical angle θc 1=arcsin(γ/ε 1). The Brewster angle θB 1 and the critical angle θc 1 are shown in Fig. 2(b) with γ changing from εxεz/ε 1 to ε 1. It can be seen that θB 1 and θc 1 become closer and closer to 90° when γε 1. Such feature is also very different from that in isotropic case.

4. Conclusion

To summarize, we have presented a detailedly theoretical analysis on omnidirectional constant transmission and the features of Brewster angles at planar interfaces associate with a uniaxial medium. Omnidirectional constant transmission, which is useful for a beam splitter and an attenuator under the situation of wide incidence, can occur at the interfaces associated with a uniaxial medium under certain conditions. The condition for omnidirectional constant transmission is much looser than for omnidirectional total transmission and quite easy to fulfill practically. The tuning character of Brewster angle at planar interfaces associated with uniaxial media can be used to steer light and also provides new methods for refracting light at any special incident angle without loss. Especially, omnidirectional constant transmission and negative Brewster angle offer mechanisms of amplitude control for negative refraction in anisotropic media. Moreover, these properties of uniaxial media give new ways of bending, polarizing, angular dispersion, energy filtering for light with extraordinary characters and offer considerable potential device applications. Such properties may also provide new experimental opportunities to investigate the physical phenomena associated with uniaxial media.

Acknowledgement

This work is supported by the National Natural Science Foundations of China (Grant Nos. 60477042 and 60878017) and Shenzhen Key Laboratory of Micro-nano Photonic Information Technology.

References and links

1. M. Born, and E. Wolf, Principles of Optics, 6th ed. (Pergamon, New York, 1980).

2. Y. Lu, P. Wang, P. Yao, J. Xie, and H. Ming, “Negative refraction at the interface of uniaxial anisotropic media,” Opt. Commun. 246(4-6), 429–435 (2005). [CrossRef]  

3. X. L. Chen, M. He, Y. X. Du, W. Y. Wang, and D. F. Zhang, “Negative refraction: an intrinsic property of uniaxial crystals,” Phys. Rev. B 72, 1–4 (2005). [CrossRef]  

4. H. L. Luo, W. Hu, X. N. Yi, H. Y. Liu, and J. Zhu, “Amphoteric refraction at the interface between isotropic and anisotropic media,” Opt. Commun. 254(4-6), 353–360 (2005). [CrossRef]  

5. L. I. Perez, M. T. Garea, and R. M. Echarri, “Isotropic-uniaxial crystal interfaces: Negative refraction and backward wave phenomena,” Opt. Commun. 254(1-3), 10–18 (2005). [CrossRef]  

6. Y. Zhang, B. Fluegel, and A. Mascarenhas, “Total negative refraction in real crystals for ballistic electrons and light,” Phys. Rev. Lett. 91(15), 157404 (2003). [CrossRef]   [PubMed]  

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8. M. Elshazly-Zaghloul and R. M. A. Azzam, “Brewster and pseudo-Brewster angles of uniaxial crystal surfaces and their use for determination of optical properties,” J. Opt. Soc. Am. 72(5), 657–661 (1982). [CrossRef]  

9. J. Lekner, “Brewster angles in reflection by uniaxial crystals,” J. Opt. Soc. Am. A 10(9), 2059–2064 (1993). [CrossRef]  

10. J. Lekner, “Reflection by uniaxial crystals: polarizing angleand Brewster angle,” J. Opt. Soc. Am. A 16(11), 2763–2766 (1999). [CrossRef]  

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13. R. A. Shelby, D. R. Smith, and S. Schultz, “Experimental verification of a negative index of refraction,” Science 292(5514), 77–79 (2001). [CrossRef]   [PubMed]  

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16. M. J. Weber, Handbook of optical materials. (CRC, New York, 2003).

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Figures (2)

Fig. 1
Fig. 1 Principal axes of the anisotropic medium (x,y,z) and the surface coordinates (x,y,z ).
Fig. 2
Fig. 2 (a)Brewster angles θB 1 and θB as functions of γ at the surface of Ba(NO3)2 (ε 1=1.57142) and calcite (εx =1.4862, εz =1.6582); (b)Brewster angle θB 1 and critical angle θc 1 as functions of γ at the same kind of surface.

Equations (27)

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x=xcosθ+z'sinθ,y=y,z=xsinθ+z'cosθ,
H=(0,H0,0),E=(kzH0/ωε0εx,0,kxH0/ωε0εz),
kx2/εz+kz2/εx=k02,
kix'=krx'=ktx'B,
αB2+βBkz'+γkz'2=k02εzεx,
α=εxcos2θ+εzsin2θ,β=(εxεz)sin2θ,γ=εxsin2θ+εzcos2θ.
kz±'=βB/2γ±A
A=[εzεx(γk02B2)]1/2/γ.
H=(0,H0,0),E=(γkz'+βB/2,0,αBβkz'/2)H0/ωε0εzεx.
Hi=(0,H0,0),Ei=(γA,0,αBβkiz'/2)H0/ωε0εzεx
Hr=r(0,H0,0),Er=r(γA,0,αBβkrz'/2)H0/ωε0εzεx
Ht=t(0,H0,0),Et=t(ktz',0,B)H0/ωε0ε1.
r=Hr/Hi=(γA/εzεxktz/ε1)/(γA/εzεx+ktz/ε1),
t=Ht/Hi=(2γA/εzεx)/(γA/εzεx+ktz/ε1).
S=Re[(αB+βkz'/2,0,γkz'+βB/2)H02/2ωε0εzεx].
tgθsi=Six'/Siz'=β/2γ+Bεxεz/Aγ2,
tgθsr=Srx'/Srz'=β/2γ+Bεxεz/Aγ2.
γ=ε1
εzεx=ε12.
r=[1/(εzεx)1/21/ε1]/[1/(εzεx)1/2+1/ε1].
Si=Re[(αB+βkiz'/2,0,γA)H02/2ωε0εzεx],
Sr=Re[(αB+βkrz'/2,0,γA)r2H02/2ωε0εzεx].
R=Jr/Ji=|r|2.
T=1|r|2
B2=(εxεzε1γ)ε1k02/(εxεzε12),
tan2θB1=(εxεzε1γ)/(ε1γε12).
tan2θB1/(tanθB2±±|β|/2γ)2=ε12/γ2.
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