Abstract
We have developed a nonperturbative analytical approach to the problem of the interaction of high-power chirped ultrashort pulses with molecular systems. We have considered a molecule with two electronic states in a solvent interacting with a strong chirped pulse, whose field amplitude can be represented in the form: , where and φ(t) are real functions of time. We consider the case when the electron-vibrational interaction can be described as a Gaussian-Markovian process.
© 1998 IEEE
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