Fast Recombination after Electron Photo-Detachment of Hydroxide in H-bonded Liquids

Hubert Rossmadl; Martin Fischer; Alfred Laubereau; Hristo Iglev

doi:10.1364/ICUSD.2012.IM3D.6

Research in Optical Sciences
OSA Technical Digest (Optica Publishing Group, 2012),
paper IM3D.6
•https://doi.org/10.1364/ICUSD.2012.IM3D.6

Fast Recombination after Electron Photo-Detachment of Hydroxide in H-bonded Liquids

Hubert Rossmadl, Martin Fischer, Alfred Laubereau, and Hristo Iglev

International Conference on Ultrafast Structural Dynamics 2012

Berlin Germany
19–21 March 2012
ISBN: 978-1-55752-939-8

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H. Rossmadl, M. Fischer, A. Laubereau, and H. Iglev, "Fast Recombination after Electron Photo-Detachment of Hydroxide in H-bonded Liquids," in Research in Optical Sciences, OSA Technical Digest (Optica Publishing Group, 2012), paper IM3D.6.

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Abstract

Femtosecond pump-repump-probe spectroscopy on OH⁻ in H-bonded liquids reveals an ultrafast (0.7–1 ps) geminate recombination channel. The process is assigned to formation of short-lieved OH:e⁻ pairs facilitated by the inhomogeneity local H-bonding environment of OH⁻.

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