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Structure and Energy Transport in Membrane-Bound Porphyrin Aggregates by Fluorescence Detected 2D Electronic Coherence Spectroscopy

Geoffrey A. Lott, James K. Utterback, Alejandro Perdomo, Alan Aspuru-Guzik, and Andrew H. Marcus

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Abstract

We studied the electronic coupling and excited state dynamics of magnesium meso tetraphenylporphyrin dimers, which self-assemble in room temperature lipid bilayer vesicles. This was accomplished using fluorescence-detected two-dimensional electronic coherence spectroscopy.

© 2010 Optical Society of America

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