Dispersion of the fifth-order nonlinear optical susceptibility 113333 (5) (;,0,0,0,0) of a polydiacetylene film

Ke Yang; Jayant Kumar; Woohong Kim; Sukant Tripathy

doi:10.1364/OTF.2001.OMC5

Organic Thin Films
OSA Trends in Optics and Photonics (Optica Publishing Group, 2001),
paper OMC5
•https://doi.org/10.1364/OTF.2001.OMC5

Dispersion of the fifth-order nonlinear optical susceptibility 113333 (5) (;,0,0,0,0) of a polydiacetylene film

Ke Yang, Jayant Kumar, Woohong Kim, and Sukant Tripathy

Organic Thin Films 2001

Long Beach, California United States
ISBN: 1-55752-685-0

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Third-Order Nonlinear Optics (OMC)

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K. Yang, J. Kumar, W. Kim, and S. Tripathy, "Dispersion of the fifth-order nonlinear optical susceptibility 113333 (5) (;,0,0,0,0) of a polydiacetylene film," in Organic Thin Films , J. Armistead, J. Heflin, A. Jen, and R. Norwood, eds., Vol. 64 of OSA Trends in Optics and Photonics (Optica Publishing Group, 2001), paper OMC5.

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Abstract

The dispersion of the fifth-order nonlinear optical susceptibility 113333 (5) (;,0,0,0,0) of a spin-coated polydiacetylene film ( poly(BPOD), i.e., poly8-butoxy carbonyl methyl urethanyl1-(5-pyrimidyl)-octa-1, 3-diyne ) is determined through electroabsorption spectroscopy. The maximum values of the real and the imaginary parts of 113333 (5) (;,0,0,0,0) are 9.8710 21 esu and 1.2810 20 esu , respectively. A model is proposed to explain the spectral dispersion of the nonlinear optical susceptibility.

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