Ultrafast Spin-State Conversion in Solvated Transition Metal Complexes Probed with Femtosecond Soft X-ray Spectroscopy

Nils Huse; Hana Cho; Hana Cho; Tae Kyu Kim; Lindsey Jamula; James K. McCusker; Frank M. F. de Groot; Robert W. Schoenlein; Robert W. Schoenlein

doi:10.1364/UP.2010.TuD2

International Conference on Ultrafast Phenomena
OSA Technical Digest (CD) (Optica Publishing Group, 2010),
paper TuD2
•https://doi.org/10.1364/UP.2010.TuD2

Ultrafast Spin-State Conversion in Solvated Transition Metal Complexes Probed with Femtosecond Soft X-ray Spectroscopy

Nils Huse, Hana Cho, Tae Kyu Kim, Lindsey Jamula, James K. McCusker, Frank M. F. de Groot, and Robert W. Schoenlein

International Conference on Ultrafast Phenomena 2010

Snowmass, Colorado United States
18–23 July 2010
ISBN: 978-1-55752-894-0

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Chemical Reaction Dynamics (TuD)

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N. Huse, H. Cho, T. K. Kim, L. Jamula, J. K. McCusker, F. M. F. de Groot, and R. W. Schoenlein, "Ultrafast Spin-State Conversion in Solvated Transition Metal Complexes Probed with Femtosecond Soft X-ray Spectroscopy," in International Conference on Ultrafast Phenomena, OSA Technical Digest (CD) (Optica Publishing Group, 2010), paper TuD2.

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Abstract

We report the first femtosecond soft x-ray spectroscopy of solvated transition-metal complexes: Structural dynamics mediate ultrafast spin-state conversion and symmetry-specific valence-charge localization. This study demonstrates the unique potential of ultrafast soft x-ray spectroscopy in solutions.

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