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Exciton-Driven Ultrafast Enhancement of Quasiparticle Bandgap and Effective Mass in Monolayer MoS2

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Abstract

We report an ultrafast increase of the quasi-particle bandgap and effective mass in photoexcited monolayer MoS2 on HOPG, utilizing extreme-ultraviolet time- and angle-resolved photoemission spectroscopy (XUV-trARPES). Combined with theoretical models, we attribute these compelling band renormalizations to the excitonic effects from bound electron-hole pairs.

© 2022 The Author(s)

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