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Momentum-Resolved Intervalley and Intravalley Exciton Coupling in Monolayer WS2

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Abstract

Using time-resolved angle-resolved photoemission spectroscopy (tr-ARPES), we image the dynamics of intervalley and intravalley excitons in monolayer WS2. We observe strong coupling between photoexcited B and A excitons and directly visualize the ultrafast valley depolarization.

© 2022 The Author(s)

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