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Optica Publishing Group
  • Frontiers in Optics + Laser Science 2023 (FiO, LS)
  • Technical Digest Series (Optica Publishing Group, 2023),
  • paper LTu6F.2

Temperature-Controlled Ultrafast Dynamics of an Antiferromagnetically Coupled Molecular Dimer

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Abstract

Two-dimensional electronic measurements reveal the role of ferromagnetic and antiferromagnetic interactions in the temperature-dependent, reversible dimerization of copper(II) hexaethyl tripyrrin-1,14-dione. Dimerization significantly alters the optical properties, with long relaxation times observed at low temperatures.

© 2023 The Author(s)

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