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Dynamic intensity borrowing induced by coherent vibrations in J-aggregates detected by sub-5-fs spectroscopy

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Abstract

Sub-5-fs real-time spectroscopy revealed that coherent molecular vibrations coupled to the Frenkel exciton system. The oscillation in the induced absorption spectrum is interpreted as the modulated transition diople moment due to the oscillator strength transfer.

© 2000 Optical Society of America

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