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Multiple scattering by random particulate media: exact 3D results

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Abstract

We use the numerically exact superposition T-matrix method to perform extensive computations of electromagnetic scattering by a 3D volume filled with randomly distributed wavelength-sized particles. These computations are used to simulate and analyze the effect of randomness of particle positions as well as the onset and evolution of various multiple-scattering effects with increasing number of particles in a statistically homogeneous volume of discrete random medium. Our exact results illustrate and substantiate the methodology underlying the microphysical theories of radiative transfer and coherent backscattering. Furthermore, we show that even in densely packed media, the light multiply scattered along strings of widely separated particles still provides a significant contribution to the total scattered signal and thereby makes quite pronounced the classical radiative transfer and coherent backscattering effects.

©2007 Optical Society of America

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Figures (11)

Fig. 1.
Fig. 1. Spherical scattering volume V filled with N randomly positioned particles.
Fig. 2.
Fig. 2. Electromagnetic scattering by a volume V of disretete random medium. In this case the scattering volume is filled with 20 randomly positioned particles.
Fig. 3.
Fig. 3. Angular distribution of scattered intensity in the far-field zone of the spherical volume V filled with N particles. (a) N = 1 and m = 1.32. (b) N = 5 and m = 1.32. (c) N = 20 and m = 1.32. (d) N = 40 and m = 1.32. (e) N = 80 and m = 1.32. (f) N = 80 and m = 1.32. (g) N = 80 and m = 1.5. (h) N = 80 and m = 1.32, random orientation. (i) N = 80 and m = 1.5, random orientation. The gray scale was individually adjusted in order to maximally reveal the details of each scattering pattern. Panel (a) also shows the angular coordinates used for all panels.
Fig. 4.
Fig. 4. Interference origin of (a) speckle and (b) coherent backscattering.
Fig. 5.
Fig. 5. Two random realizations of the 80-particle group created with (a) RCG-1 and (b) RCG-2.
Fig. 6.
Fig. 6. Elements of the normalized Stokes scattering matrix computed for the volume V of discrete random medium filled with N = 1, …,240 particles having the same refractive index m = 1.32.
Fig. 7.
Fig. 7. Elements of the normalized Stokes scattering matrix computed for the volume V of discrete random medium filled with N = 1, …, 160 particles having the same refractive index m = 1.5.
Fig. 8.
Fig. 8. Elements of the normalized Stokes scattering matrix computed for the volume V of discrete random medium filled with a varying number of particles. (a) m = 1.32 (solid curves) and 1.5 (dotted curve). (b) – (d) m = 1.32. (e) and (f) m = 1.5.
Fig. 9.
Fig. 9. Forward-scattering interference.
Fig. 10.
Fig. 10. Polarization characteristics of backscattered light computed for the volume V of discrete random medium filled with N = 1, …, 240 particles having the same refractive index m = 1.32.
Fig. 11.
Fig. 11. Polarization characteristics of backscattered light computed for the volume V of discrete random medium filled with N = 1, …, 160 particles having the same refractive index m = 1.5.

Equations (10)

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I sca Q sca U sca V sca Z n ̂ sca n ̂ inc I inc Q inc U inc V inc .
[ a 1 ( Θ ) b 1 ( Θ ) 0 0 b 1 ( Θ ) a 2 ( Θ ) 0 0 0 0 a 3 ( Θ ) b 2 ( Θ ) 0 0 b 2 ( Θ ) a 4 ( Θ ) ] .
1 2 0 π d Θ sin Θ a 1 ( Θ ) = 1 .
Δ = k 1 ( r n r 1 ) ( n ̂ inc + n ̂ sca ) .
1 2 ( I sca + Q sca ) 1 2 [ a 1 ( Θ ) + 2 b 1 ( Θ ) + a 2 ( Θ ) ] ,
1 2 ( I sca Q sca ) 1 2 [ a 1 ( Θ ) a 2 ( Θ ) ] ,
1 2 ( I sca + V sca ) 1 2 [ a 1 ( Θ ) + a 4 ( Θ ) ] ,
1 2 ( I sca V sca ) 1 2 [ a 1 ( Θ ) a 4 ( Θ ) ] ,
μ L = I sca Q sca I sca + Q sca = a 1 ( Θ ) a 2 ( Θ ) a 1 ( Θ ) + 2 b 1 ( Θ ) + a 2 ( Θ ) ,
μ C = I sca + V sca I sca V sca = a 1 ( Θ ) + a 4 ( Θ ) a 1 ( Θ ) a 4 ( Θ ) .
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