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Excitonic Optical Nonlinearity in Semiconductor Quantum Spheres

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Abstract

It is numerically confirmed that the third-order optical susceptibility χ(3)(ω;–ω,ω,–ω) is enhanced by the mesoscopically enhanced transition dipole moment of excitons in CuCl quantum spheres (QS's) but it is not in GaAs QS's and it is marginal for CdS QS's.

© 1989 Optical Society of America

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